#------------------------------------------------------------------------------ #$Date: 2011-09-10 04:16:28 +0100 (Sat, 10 Sep 2011) $ #$Revision: 25271 $ #$URL: svn://www.crystallography.net/cod/cif/2/2005580.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2005580 loop_ _publ_author_name 'Long, D.-L.' 'Xin, X.-Q.' 'Huang, X.-Y.' _publ_contact_author ; Xin-quan Xin State Key Laboratory of Coordination Chemistry Coordination Chemistry Institute Nanjing University Nanjing 210093 P. R. China ; _publ_section_title ; (Dimercaptomethylenepropanedinitrilato-S,S')(pyridine)(triphenylphosphine)palladium(II)--Acetonitrile (1/1) ; _journal_issue 11 _journal_name_full 'Acta Crystallographica Section C' _journal_page_first 2724 _journal_page_last 2726 _journal_volume 52 _journal_year 1996 _chemical_formula_iupac '[Pd (C4 N2 S2) (C5 H5 N) (C18 H15 P)]' _chemical_formula_moiety 'C27 H20 N3 P Pd S2, C2 H3 N' _chemical_formula_sum 'C29 H23 N4 P Pd S2' _chemical_formula_weight 629.02 _space_group_IT_number 2 _symmetry_cell_setting triclinic _symmetry_space_group_name_Hall '-P 1' _symmetry_space_group_name_H-M 'P -1' _atom_type_scat_source IntTabIV _cell_angle_alpha 93.56(2) _cell_angle_beta 94.94(2) _cell_angle_gamma 94.31(3) _cell_formula_units_Z 2 _cell_length_a 9.7330(10) _cell_length_b 10.601(6) _cell_length_c 13.835(4) _cell_measurement_reflns_used 25 _cell_measurement_temperature 296 _cell_measurement_theta_max 14.93 _cell_measurement_theta_min 14.06 _cell_volume 1414.8(9) _computing_cell_refinement 'CAD-4 Software' _computing_data_collection 'CAD-4 Software (Enraf-Nonius, 1989)' _computing_data_reduction TEXSAN _computing_molecular_graphics 'ORTEPII (Johnson, 1976), PLUTO (Motherwell & Clegg, 1978)' _computing_structure_refinement TEXSAN _computing_structure_solution 'MITHRIL (Gilmore, 1983)' _diffrn_measurement_device 'Enraf-Nonius CAD-4' _diffrn_measurement_method '\w/2\q scans' _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_limit_h_max 11 _diffrn_reflns_limit_h_min 0 _diffrn_reflns_limit_k_max 12 _diffrn_reflns_limit_k_min -12 _diffrn_reflns_limit_l_max 16 _diffrn_reflns_limit_l_min -16 _diffrn_reflns_number 4979 _diffrn_reflns_theta_max 25 _diffrn_standards_decay_% 1.1 _diffrn_standards_interval_count 300 _diffrn_standards_number 3 _exptl_absorpt_coefficient_mu 0.868 _exptl_absorpt_correction_T_max 0.88 _exptl_absorpt_correction_T_min 0.73 _exptl_absorpt_correction_type 'empirical, \y scans (TEXSAN; Molecular Structure Corporation, 1987)' _exptl_crystal_colour orange _exptl_crystal_density_diffrn 1.48 _exptl_crystal_density_meas 'not measured' _exptl_crystal_description Needle _exptl_crystal_size_max 0.90 _exptl_crystal_size_mid 0.25 _exptl_crystal_size_min 0.15 _refine_diff_density_max 0.88 _refine_diff_density_min -1.12 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_obs 1.35 _refine_ls_hydrogen_treatment 'H atoms: see text' _refine_ls_number_parameters 334 _refine_ls_number_reflns 4417 _refine_ls_R_factor_obs 0.037 _refine_ls_shift/esd_max 0.05 _refine_ls_structure_factor_coef F _refine_ls_weighting_scheme ' w=1/\s^2^(F)' _refine_ls_wR_factor_obs 0.048 _reflns_number_observed 4417 _reflns_number_total 4979 _reflns_observed_criterion I>3\s(I) _[local]_cod_data_source_file bm1065.cif _[local]_cod_data_source_block default _cod_depositor_comments ; The following automatic conversions were performed: '_symmetry_cell_setting' value 'Triclinic' changed to 'triclinic' according to /home/saulius/struct/CIF-dictionaries/cif_core.dic dictionary named 'cif_core.dic' version 2.4.1 from 2010-06-29. Automatic conversion script Id: cif_fix_values 1715 2011-07-08 13:25:40Z adriana ; _cod_original_cell_volume 1415(2) _cod_database_code 2005580 loop_ _symmetry_equiv_pos_as_xyz x,y,z -x,-y,-z loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 _atom_site_aniso_type_symbol Pd .0370(2) .0420(2) .0333(2) .00190(10) .00300(10) .00370(10) Pd S1 .0605(6) .0482(5) .0413(5) .0019(4) .0088(4) .0081(4) S S2 .0683(6) .0580(6) .0391(5) .0013(4) .0137(4) .0007(4) S P .0338(4) .0411(5) .0345(4) .0017(4) .0045(3) .0049(3) P N1 .040(2) .046(2) .0380(10) .0060(10) -.0020(10) .0030(10) N N2 .083(3) .075(3) .084(3) .022(2) .024(2) .025(2) N N3 .092(3) .099(3) .068(3) .020(2) .036(2) .020(2) N C1 .039(2) .050(2) .055(2) .005(2) -.002(2) .003(2) C C2 .050(2) .053(2) .072(3) -.005(2) -.002(2) .006(2) C C3 .071(3) .046(2) .081(3) .000(2) -.005(2) .005(2) C C4 .063(3) .061(3) .079(3) .025(2) -.002(2) .001(2) C C5 .040(2) .060(2) .060(2) .009(2) .002(2) .001(2) C C6 .035(2) .062(2) .042(2) .007(2) .0040(10) .009(2) C C7 .041(2) .069(3) .047(2) .010(2) .010(2) .018(2) C C8 .048(2) .074(3) .058(2) .015(2) .015(2) .025(2) C C9 .052(2) .068(3) .058(2) .007(2) .016(2) .024(2) C C21 .036(2) .042(2) .044(2) .0040(10) .0100(10) .0070(10) C C22 .055(2) .051(2) .050(2) .010(2) .007(2) .003(2) C C23 .074(3) .056(2) .064(3) .016(2) .019(2) -.002(2) C C24 .062(2) .056(2) .081(3) .021(2) .023(2) .019(2) C C25 .045(2) .065(3) .072(3) .015(2) .009(2) .025(2) C C26 .042(2) .052(2) .050(2) .004(2) .005(2) .009(2) C C31 .036(2) .042(2) .036(2) .0020(10) .0040(10) .0060(10) C C32 .047(2) .061(2) .039(2) .001(2) .008(2) .008(2) C C33 .061(3) .072(3) .039(2) -.002(2) -.008(2) .002(2) C C34 .044(2) .088(3) .060(3) -.002(2) -.009(2) .000(2) C C35 .039(2) .104(4) .062(3) -.014(2) .008(2) .004(2) C C36 .046(2) .070(3) .041(2) -.005(2) .006(2) .006(2) C C41 .040(2) .048(2) .035(2) -.0040(10) .0020(10) .0040(10) C C42 .043(2) .073(3) .064(2) .001(2) .011(2) .017(2) C C43 .052(3) .096(4) .079(3) -.016(2) .018(2) .023(3) C C44 .081(3) .072(3) .063(3) -.021(3) .006(2) .025(2) C C45 .080(3) .051(2) .058(2) -.007(2) -.005(2) .016(2) C C46 .052(2) .050(2) .047(2) -.002(2) -.001(2) .009(2) C N4 .114(5) .149(5) .114(5) -.026(4) .033(4) -.031(4) C C10 .111(5) .112(5) .107(5) -.016(4) .036(4) .016(4) C C11 .097(4) .091(4) .085(4) -.019(3) .040(3) -.015(3) C loop_ _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z Pd .22769(3) .03259(2) .07635(2) S1 .26910(10) .23810(9) .03820(6) S2 .28190(10) .01720(10) -.08529(7) P .20458(9) .08660(8) .23738(6) N1 .1921(3) -.1621(3) .0864(2) N2 .3654(4) .4975(4) -.1228(3) N3 .4318(5) .1614(4) -.3049(3) C1 .0679(4) -.2152(3) .1034(3) C2 .0423(4) -.3439(4) .1094(3) C3 .1472(5) -.4206(4) .0990(3) C4 .2746(5) -.3668(4) .0813(3) C5 .2951(4) -.2381(4) .0756(3) C6 .3062(3) .1797(4) -.0749(3) C7 .3488(4) .2552(4) -.1466(3) C8 .3578(4) .3889(4) -.1329(3) C9 .3929(4) .2012(4) -.2336(3) C21 .1018(3) .2225(3) .2533(2) C22 .1193(4) .3032(4) .3367(3) C23 .0325(5) .4000(4) .3478(3) C24 -.0705(5) .4159(4) .2765(3) C25 -.0881(4) .3361(4) .1933(3) C26 -.0018(4) .2392(3) .1814(3) C31 .3727(3) .1258(3) .3043(2) C32 .3914(4) .1282(4) .4053(2) C33 .5215(4) .1573(4) .4532(3) C34 .6330(4) .1833(5) .4019(3) C35 .6158(4) .1815(5) .3028(3) C36 .4863(4) .1523(4) .2536(3) C41 .1235(3) -.0355(3) .3051(2) C42 -.0114(4) -.0319(4) .3297(3) C43 -.0706(5) -.1316(5) .3777(4) C44 .0021(5) -.2334(5) .3981(3) C45 .1341(5) -.2383(4) .3728(3) C46 .1963(4) -.1398(4) .3269(3) N4 .2955(7) .4466(6) .5565(5) C10 .5278(7) .5003(6) .6547(5) C11 .3964(7) .4700(6) .5997(4) H1 -.0049 -.1620 .1117 H2 -.0476 -.3788 .1205 H3 .1323 -.5096 .1047 H4 .3485 -.4191 .0725 H5 .3839 -.2017 .0636 H6 .1907 .2926 .3863 H7 .0437 .4550 .4054 H8 -.1296 .4830 .2842 H9 -.1593 .3472 .1436 H10 -.0138 .1847 .1239 H11 .3144 .1096 .4415 H12 .5334 .1593 .5223 H13 .7227 .2024 .4350 H14 .6933 .2013 .2675 H15 .4758 .1501 .1845 H16 -.0633 .0378 .3137 H17 -.1620 -.1284 .3963 H18 -.0397 -.3008 .4308 H19 .1837 -.3100 .3865 H20 .2888 -.1429 .3103 H21 .5763 .4256 .6584 H22 .5807 .5624 .6242 H23 .5140 .5318 .7188 loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle _geom_angle_publ_flag N1 Pd S1 170.38(8) yes N1 Pd S2 95.13(8) yes N1 Pd P 95.57(8) yes S1 Pd P 94.04(4) yes S1 Pd S2 75.35(4) yes S2 Pd P 167.89(3) yes C6 S1 Pd 87.70(10) yes C6 S2 Pd 86.20(10) yes C31 P C41 104.00(10) no C31 P C21 107.9(2) no C31 P Pd 110.80(10) no C41 P C21 104.9(2) no C41 P Pd 116.30(10) no C21 P Pd 112.30(10) no C1 N1 C5 118.3(3) no C1 N1 Pd 121.7(2) no C5 N1 Pd 120.0(2) no N1 C1 C2 122.4(3) no C3 C2 C1 119.2(4) no C2 C3 C4 118.7(4) no C5 C4 C3 120.1(4) no N1 C5 C4 121.4(4) no C7 C6 S2 125.5(3) no C7 C6 S1 123.8(3) no S2 C6 S1 110.6(2) yes C6 C7 C8 121.2(4) yes C6 C7 C9 121.0(4) yes C8 C7 C9 117.7(3) yes N2 C8 C7 179.2(5) yes N3 C9 C7 177.4(5) yes C26 C21 C22 119.8(3) no C26 C21 P 118.0(3) no C22 C21 P 122.1(3) no C21 C22 C23 119.7(4) no C24 C23 C22 120.3(4) no C23 C24 C25 120.2(4) no C24 C25 C26 120.0(4) no C21 C26 C25 120.0(4) no C36 C31 C32 118.8(3) no C36 C31 P 119.1(3) no C32 C31 P 122.1(3) no C33 C32 C31 120.2(3) no C34 C33 C32 120.4(3) no C35 C34 C33 119.9(4) no C34 C35 C36 120.5(4) no C31 C36 C35 120.2(3) no C42 C41 C46 119.3(3) no C42 C41 P 122.0(3) no C46 C41 P 118.6(3) no C41 C42 C43 119.5(4) no C44 C43 C42 120.4(4) no C45 C44 C43 120.3(4) no C44 C45 C46 120.5(4) no C45 C46 C41 120.0(4) no N4 C11 C10 179.4(6) no H1 C1 N1 118.71 no H1 C1 C2 118.86 no H2 C2 C3 120.51 no H2 C2 C1 120.34 no H3 C3 C2 120.47 no H3 C3 C4 120.87 no H4 C4 C5 120.04 no H4 C4 C3 119.83 no H5 C5 N1 119.22 no H5 C5 C4 119.42 no H6 C22 C21 120.26 no H6 C22 C23 120.04 no H7 C23 C24 119.84 no H7 C23 C22 119.82 no H8 C24 C23 120.08 no H8 C24 C25 119.76 no H9 C25 C24 120.24 no H9 C25 C26 119.76 no H10 C26 C21 120.12 no H10 C26 C25 119.87 no H11 C32 C33 119.92 no H11 C32 C31 119.92 no H12 C33 C34 119.89 no H12 C33 C32 119.75 no H13 C34 C35 119.90 no H13 C34 C33 120.16 no H14 C35 C34 119.63 no H14 C35 C36 119.85 no H15 C36 C31 119.96 no H15 C36 C35 119.81 no H16 C42 C41 120.21 no H16 C42 C43 120.31 no H17 C43 C44 119.79 no H17 C43 C42 119.76 no H18 C44 C45 120.14 no H18 C44 C43 119.56 no H19 C45 C44 119.83 no H19 C45 C46 119.71 no H20 C46 C45 120.18 no H20 C46 C41 119.82 no H22 C10 H23 109.60 no H22 C10 H21 109.35 no H22 C10 C11 109.94 no H23 C10 H21 108.95 no H23 C10 C11 109.69 no H21 C10 C11 109.29 no loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_distance _geom_bond_publ_flag Pd N1 2.082(3) yes Pd S1 2.288(2) yes Pd S2 2.3400(10) yes Pd P 2.3000(10) yes S1 C6 1.724(4) yes S2 C6 1.716(4) yes P C31 1.816(3) yes P C41 1.817(3) yes P C21 1.828(3) yes N1 C1 1.341(5) yes N1 C5 1.344(5) yes N2 C8 1.146(6) yes N3 C9 1.154(5) yes C1 C2 1.377(6) no C2 C3 1.363(6) no C3 C4 1.373(6) no C4 C5 1.372(6) no C6 C7 1.385(5) yes C7 C8 1.414(6) yes C7 C9 1.414(6) yes C21 C26 1.383(5) no C21 C22 1.384(5) no C22 C23 1.387(5) no C23 C24 1.372(6) no C24 C25 1.377(6) no C25 C26 1.385(5) no C31 C36 1.381(5) no C31 C32 1.392(5) no C32 C33 1.381(5) no C33 C34 1.368(6) no C34 C35 1.365(6) no C35 C36 1.384(6) no C41 C42 1.387(5) no C41 C46 1.391(5) no C42 C43 1.397(6) no C43 C44 1.365(7) no C44 C45 1.365(7) no C45 C46 1.383(5) no N4 C11 1.108(8) no C10 C11 1.430(10) no C1 H1 .948 no C2 H2 .953 no C3 H3 .953 no C4 H4 .953 no C5 H5 .953 no C22 H6 .952 no C23 H7 .951 no C24 H8 .954 no C25 H9 .952 no C26 H10 .948 no C32 H11 .952 no C33 H12 .952 no C34 H13 .952 no C35 H14 .951 no C36 H15 .951 no C42 H16 .953 no C43 H17 .949 no C44 H18 .952 no C45 H19 .952 no C46 H20 .951 no C10 H23 .947 no C10 H22 .952 no C10 H21 .955 no loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion _geom_torsion_publ_flag Pd N1 C1 C2 179.4(3) no Pd N1 C5 C4 -179.6(3) no Pd S1 C6 C7 -177.8(3) no Pd S1 C6 S2 2.4(2) no Pd P C31 C36 16.7(3) no Pd P C31 C32 -162.2(3) no Pd P C41 C42 -105.0(3) no Pd P C41 C46 70.7(3) no Pd P C21 C26 31.1(3) no Pd P C21 C22 -152.8(3) no Pd S2 C6 C7 177.9(3) no Pd S2 C6 S1 -2.4(2) no S1 C6 C7 C8 -3.5(5) no S1 C6 C7 C9 172.6(3) no S1 Pd N1 C1 -109.7(5) no S1 Pd N1 C5 70.2(6) no S1 Pd P C31 -77.60(10) no S1 Pd P C41 163.90(10) no S1 Pd P C21 43.10(10) no S1 Pd S2 C6 1.70(10) no S2 C6 C7 C8 176.2(3) no S2 C6 C7 C9 -7.7(5) no S2 Pd N1 C1 -117.7(3) no S2 Pd N1 C5 62.2(3) no S2 Pd S1 C6 -1.70(10) no S2 Pd P C31 -49.2(2) no S2 Pd P C41 -167.6(2) no S2 Pd P C21 71.5(2) no P C31 C36 C35 -179.5(3) no P C31 C32 C33 179.4(3) no P C41 C42 C43 176.9(3) no P C41 C46 C45 -175.9(3) no P C21 C26 C25 175.8(3) no P C21 C22 C23 -175.8(3) no P Pd N1 C1 68.0(3) no P Pd N1 C5 -112.1(3) no P Pd S1 C6 172.40(10) no P Pd S2 C6 -27.6(2) no N1 C1 C2 C3 .9(6) no N1 C5 C4 C3 -.5(7) no N1 Pd S1 C6 -10.0(5) no N1 Pd P C31 102.80(10) no N1 Pd P C41 -15.7(2) no N1 Pd P C21 -136.50(10) no N1 Pd S2 C6 -179.7(2) no N2 C8 C7 C6 -172.4(2) no N2 C8 C7 C9 11.3(2) no C1 N1 C5 C4 .3(7) no C1 C2 C3 C4 -1.0(6) no C2 C3 C4 C5 .9(7) no C2 C1 N1 C5 -.5(6) no C21 C26 C25 C24 .2(7) no C21 C22 C23 C24 0(2) no C21 P C31 C36 -106.6(3) no C21 P C31 C32 74.4(3) no C21 P C41 C42 19.7(4) no C21 P C41 C46 -164.6(3) no C22 C21 C26 C25 -.3(7) no C22 C21 P C31 -30.4(3) no C22 C21 P C41 80.0(3) no C22 C23 C24 C25 -.2(8) no C23 C24 C25 C26 .1(8) no C23 C22 C21 C26 .0(10) no C26 C21 P C31 153.6(3) no C26 C21 P C41 -96.0(3) no C31 C36 C35 C34 .6(7) no C31 C32 C33 C34 -.4(8) no C31 P C41 C42 132.9(3) no C31 P C41 C46 -51.4(3) no C32 C33 C34 C35 .5(8) no C32 C31 C36 C35 -.5(6) no C32 C31 P C41 -36.6(3) no C33 C34 C35 C36 -.6(8) no C33 C32 C31 C36 .4(6) no C36 C31 P C41 142.4(3) no C41 C42 C43 C44 -1.7(7) no C41 C46 C45 C44 -.9(6) no C42 C41 C46 C45 .0(10) no C42 C43 C44 C45 .7(8) no C43 C44 C45 C46 .5(7) no C43 C42 C41 C46 1.3(6) no