#------------------------------------------------------------------------------ #$Date: 2015-04-02 12:22:18 +0100 (Thu, 02 Apr 2015) $ #$Revision: 134621 $ #$URL: svn://www.crystallography.net/cod/cif/2/00/82/2008246.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2008246 loop_ _publ_author_name 'Thangarasu Pandiyan' 'Bern\`es, Sylvain' 'Dur\'an de Baz\'ua, Carmen' _publ_section_title Dichloro[2,2'-(2,5-dithiahexamethylene)dipyridine-N,N',S,S']nickel(II) _journal_issue 3 _journal_name_full 'Acta Crystallographica Section C' _journal_page_first 318 _journal_page_last 320 _journal_paper_doi 10.1107/S010827019801422X _journal_volume 55 _journal_year 1999 _chemical_formula_iupac '[Ni Cl2(C14 H16 N2 S2 )]' _chemical_formula_moiety '[Ni(C14 H16 N2 S2 )]Cl2 ' _chemical_formula_sum 'C14 H16 Cl2 N2 Ni S2' _chemical_formula_weight 406.02 _space_group_IT_number 60 _symmetry_cell_setting orthorhombic _symmetry_space_group_name_Hall '-P 2n 2ab' _symmetry_space_group_name_H-M 'P b c n' _audit_creation_method SHELXL-97 _cell_angle_alpha 90.00 _cell_angle_beta 90.00 _cell_angle_gamma 90.00 _cell_formula_units_Z 4 _cell_length_a 14.5297(16) _cell_length_b 8.2314(14) _cell_length_c 14.3684(18) _cell_measurement_reflns_used 39 _cell_measurement_temperature 293(2) _cell_measurement_theta_max 12.49 _cell_measurement_theta_min 4.87 _cell_volume 1718.5(4) _computing_cell_refinement XSCANS _computing_data_collection 'XSCANS (Fait, 1991)' _computing_data_reduction XSCANS _computing_molecular_graphics 'SHELXTL (Sheldrick, 1995)' _computing_publication_material SHELX97 _computing_structure_refinement SHELX97 _computing_structure_solution 'SHELX97 (Sheldrick, 1997)' _diffrn_ambient_temperature 293(2) _diffrn_measured_fraction_theta_full 0.877 _diffrn_measured_fraction_theta_max 0.877 _diffrn_measurement_device_type 'Siemens P4' _diffrn_measurement_method '2\q/\w scans' _diffrn_radiation_monochromator graphite _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_av_R_equivalents 0.0183 _diffrn_reflns_av_sigmaI/netI 0.0265 _diffrn_reflns_limit_h_max 19 _diffrn_reflns_limit_h_min -1 _diffrn_reflns_limit_k_max 10 _diffrn_reflns_limit_k_min -1 _diffrn_reflns_limit_l_max 18 _diffrn_reflns_limit_l_min -1 _diffrn_reflns_number 2702 _diffrn_reflns_theta_full 27.99 _diffrn_reflns_theta_max 27.99 _diffrn_reflns_theta_min 2.80 _diffrn_standards_decay_% 6.85 _diffrn_standards_interval_count 97 _diffrn_standards_number 3 _exptl_absorpt_coefficient_mu 1.676 _exptl_absorpt_correction_T_max 0.278 _exptl_absorpt_correction_T_min 0.251 _exptl_absorpt_correction_type psi-scan _exptl_absorpt_process_details '(Fait, 1991)' _exptl_crystal_colour green _exptl_crystal_density_diffrn 1.569 _exptl_crystal_density_method 'not measured' _exptl_crystal_description prism _exptl_crystal_F_000 832 _exptl_crystal_size_max 0.6 _exptl_crystal_size_mid 0.3 _exptl_crystal_size_min 0.3 _refine_diff_density_max 0.245 _refine_diff_density_min -0.322 _refine_ls_extinction_coef 0.0053(3) _refine_ls_extinction_method SHELXL _refine_ls_goodness_of_fit_ref 1.013 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 97 _refine_ls_number_reflns 2066 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.013 _refine_ls_R_factor_all 0.0445 _refine_ls_R_factor_gt 0.0300 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w = 1/[\s^2^(Fo^2^)+(0.0206P)^2^+1.0130P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_obs 0.0641 _refine_ls_wR_factor_ref 0.0694 _reflns_number_gt 1616 _reflns_number_total 2066 _reflns_threshold_expression I>2\s(I) _[local]_cod_data_source_file fg1490.cif _[local]_cod_data_source_block tp5 _[local]_cod_cif_authors_sg_H-M Pbcn _cod_depositor_comments ; The following automatic conversions were performed: '_symmetry_cell_setting' value 'Orthorhombic' changed to 'orthorhombic' according to '/home/saulius/struct/CIF-dictionaries/cif_core.dic' dictionary named 'cif_core.dic' version 2.4.1 from 2010-06-29. Automatic conversion script Id: cif_fix_enum 1527 2010-12-29 10:47:43Z saulius The following automatic conversions were performed: '_refine_ls_weighting_scheme' value 'calc w = 1/[\s^2^(Fo^2^)+(0.0206P)^2^+1.0130P] where P=(Fo^2^+2Fc^2^)/3' was changed to 'calc'. New tag '_refine_ls_weighting_details' was created. The value of the new tag was set to 'w = 1/[\s^2^(Fo^2^)+(0.0206P)^2^+1.0130P] where P=(Fo^2^+2Fc^2^)/3'. Automatic conversion script Id: cif_fix_values 3143 2015-03-26 13:38:13Z robertas ; _cod_database_code 2008246 loop_ _symmetry_equiv_pos_as_xyz 'x, y, z' '-x+1/2, -y+1/2, z+1/2' '-x, y, -z+1/2' 'x+1/2, -y+1/2, -z' '-x, -y, -z' 'x-1/2, y-1/2, -z-1/2' 'x, -y, z-1/2' '-x-1/2, y-1/2, z' loop_ _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_refinement_flags _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group _atom_site_type_symbol Ni1 0.5000 0.24074(4) 0.2500 0.02683(11) Uani d S 1 . . Ni Cl1 0.42223(4) 0.04683(7) 0.34507(4) 0.04086(14) Uani d . 1 . . Cl S1 0.42148(5) 0.45514(8) 0.33515(4) 0.05032(17) Uani d . 1 . . S N1 0.38552(11) 0.2680(2) 0.16125(11) 0.0332(4) Uani d . 1 . . N C1 0.4490(2) 0.6277(3) 0.2609(2) 0.0719(9) Uani d . 1 . . C H1A 0.4139 0.6211 0.2036 0.108 Uiso calc R 1 . . H H1B 0.4325 0.7280 0.2923 0.108 Uiso calc R 1 . . H C2 0.30961(16) 0.3965(3) 0.29291(17) 0.0534(7) Uani d . 1 . . C H2A 0.2864 0.3086 0.3312 0.064 Uiso calc R 1 . . H H2B 0.2679 0.4878 0.2997 0.064 Uiso calc R 1 . . H C3 0.30933(14) 0.3429(3) 0.19313(15) 0.0373(5) Uani d . 1 . . C C4 0.23288(16) 0.3673(3) 0.13748(18) 0.0492(6) Uani d . 1 . . C H4A 0.1809 0.4183 0.1614 0.059 Uiso calc R 1 . . H C5 0.23435(18) 0.3153(3) 0.04624(18) 0.0561(7) Uani d . 1 . . C H5A 0.1836 0.3306 0.0078 0.067 Uiso calc R 1 . . H C6 0.31263(18) 0.2401(3) 0.01305(17) 0.0511(6) Uani d . 1 . . C H6A 0.3156 0.2046 -0.0483 0.061 Uiso calc R 1 . . H C7 0.38624(16) 0.2184(3) 0.07194(15) 0.0395(5) Uani d . 1 . . C H7A 0.4387 0.1673 0.0491 0.047 Uiso calc R 1 . . H loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Ni1 0.02577(17) 0.02649(17) 0.02823(17) 0.000 0.00156(13) 0.000 Cl1 0.0405(3) 0.0411(3) 0.0410(3) -0.0123(2) 0.0048(2) 0.0039(2) S1 0.0568(4) 0.0486(3) 0.0455(3) 0.0166(3) -0.0045(3) -0.0167(3) N1 0.0308(8) 0.0366(9) 0.0322(8) 0.0038(7) -0.0012(7) 0.0014(7) C1 0.088(2) 0.0275(10) 0.101(2) 0.0115(12) -0.019(2) -0.0075(15) C2 0.0418(13) 0.0687(17) 0.0498(13) 0.0216(12) 0.0055(11) -0.0058(13) C3 0.0315(10) 0.0390(11) 0.0413(11) 0.0048(9) 0.0012(9) 0.0032(10) C4 0.0351(11) 0.0493(13) 0.0633(15) 0.0095(10) -0.0053(11) 0.0084(12) C5 0.0489(14) 0.0601(15) 0.0592(15) 0.0065(13) -0.0244(12) 0.0068(14) C6 0.0553(14) 0.0570(15) 0.0410(12) 0.0010(13) -0.0127(11) 0.0006(12) C7 0.0405(11) 0.0427(12) 0.0353(10) 0.0036(9) -0.0018(9) -0.0008(9) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0033 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0061 0.0033 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' S S 0.1246 0.1234 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Cl Cl 0.1484 0.1585 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Ni Ni 0.3393 1.1124 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag N1 Ni1 N1 . 3_655 167.79(9) y N1 Ni1 Cl1 . . 92.51(5) y N1 Ni1 Cl1 3_655 . 95.65(5) n N1 Ni1 Cl1 . 3_655 95.65(5) y N1 Ni1 Cl1 3_655 3_655 92.51(5) n Cl1 Ni1 Cl1 . 3_655 96.00(3) y N1 Ni1 S1 . 3_655 89.35(5) y N1 Ni1 S1 3_655 3_655 81.78(5) n Cl1 Ni1 S1 . 3_655 174.85(2) y Cl1 Ni1 S1 3_655 3_655 88.58(2) n N1 Ni1 S1 . . 81.78(5) y N1 Ni1 S1 3_655 . 89.35(5) n Cl1 Ni1 S1 . . 88.58(2) y Cl1 Ni1 S1 3_655 . 174.85(2) n S1 Ni1 S1 3_655 . 86.94(4) y C2 S1 C1 . . 102.10(13) y C2 S1 Ni1 . . 93.41(8) y C1 S1 Ni1 . . 99.72(10) y C7 N1 C3 . . 117.97(18) n C7 N1 Ni1 . . 122.56(14) n C3 N1 Ni1 . . 119.43(13) n C1 C1 S1 3_655 . 109.64(18) n C3 C2 S1 . . 113.78(17) n N1 C3 C4 . . 122.0(2) n N1 C3 C2 . . 117.21(19) n C4 C3 C2 . . 120.8(2) n C5 C4 C3 . . 119.5(2) n C4 C5 C6 . . 118.7(2) n C7 C6 C5 . . 119.1(2) n N1 C7 C6 . . 122.7(2) n loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag Ni1 N1 . 2.1078(16) y Ni1 N1 3_655 2.1078(16) n Ni1 Cl1 . 2.3855(6) y Ni1 Cl1 3_655 2.3855(6) n Ni1 S1 3_655 2.4316(7) n Ni1 S1 . 2.4316(7) y S1 C2 . 1.801(3) y S1 C1 . 1.821(3) y N1 C7 . 1.347(3) n N1 C3 . 1.348(3) n C1 C1 3_655 1.516(6) n C2 C3 . 1.500(3) n C3 C4 . 1.383(3) n C4 C5 . 1.379(4) n C5 C6 . 1.380(4) n C6 C7 . 1.375(3) n loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_site_symmetry_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA C1 H1B Cl1 1_565 0.97 2.74 3.676(3) 163 loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_4 _geom_torsion N1 Ni1 S1 C2 . . 27.15(10) N1 Ni1 S1 C2 3_655 . -161.27(10) Cl1 Ni1 S1 C2 . . -65.60(9) Cl1 Ni1 S1 C2 3_655 . 87.5(3) S1 Ni1 S1 C2 3_655 . 116.93(9) N1 Ni1 S1 C1 . . -75.76(11) N1 Ni1 S1 C1 3_655 . 95.83(11) Cl1 Ni1 S1 C1 . . -168.50(10) Cl1 Ni1 S1 C1 3_655 . -15.4(3) S1 Ni1 S1 C1 3_655 . 14.03(10) N1 Ni1 N1 C7 3_655 . 115.48(16) Cl1 Ni1 N1 C7 . . -112.54(16) Cl1 Ni1 N1 C7 3_655 . -16.25(17) S1 Ni1 N1 C7 3_655 . 72.26(16) S1 Ni1 N1 C7 . . 159.26(17) N1 Ni1 N1 C3 3_655 . -62.07(15) Cl1 Ni1 N1 C3 . . 69.91(15) Cl1 Ni1 N1 C3 3_655 . 166.20(15) S1 Ni1 N1 C3 3_655 . -105.29(15) S1 Ni1 N1 C3 . . -18.29(15) C2 S1 C1 C1 . 3_655 -143.7(3) Ni1 S1 C1 C1 . 3_655 -48.1(3) C1 S1 C2 C3 . . 62.4(2) Ni1 S1 C2 C3 . . -38.28(18) C7 N1 C3 C4 . . 1.0(3) Ni1 N1 C3 C4 . . 178.63(17) C7 N1 C3 C2 . . 179.7(2) Ni1 N1 C3 C2 . . -2.7(3) S1 C2 C3 N1 . . 32.2(3) S1 C2 C3 C4 . . -149.1(2) N1 C3 C4 C5 . . -0.7(4) C2 C3 C4 C5 . . -179.4(2) C3 C4 C5 C6 . . 0.0(4) C4 C5 C6 C7 . . 0.5(4) C3 N1 C7 C6 . . -0.5(3) Ni1 N1 C7 C6 . . -178.08(18) C5 C6 C7 N1 . . -0.2(4)