#------------------------------------------------------------------------------ #$Date: 2016-02-14 04:40:26 +0000 (Sun, 14 Feb 2016) $ #$Revision: 176432 $ #$URL: svn://www.crystallography.net/cod/cif/2/01/16/2011644.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2011644 loop_ _publ_author_name 'Virovets, Alexander V.' 'Kalinina, Irina V.' 'Fedin, Vladimir P.' 'Fenske, Dieter' _publ_section_title ;Tetragonal polymorphic modification of tetrakis(N,N-diethyldithiocarbamato-S,S')tellurium(IV) ; _journal_issue 12 _journal_name_full 'Acta Crystallographica Section C' _journal_page_first e589 _journal_page_last e590 _journal_paper_doi 10.1107/S0108270100015389 _journal_volume 56 _journal_year 2000 _chemical_formula_structural 'C20 H40 N4 S8 Te' _chemical_formula_sum 'C20 H40 N4 S8 Te' _chemical_formula_weight 720.64 _chemical_name_common none _chemical_name_systematic ; tetracis(diethyldithiocarbamato)tellurium(IV) ; _space_group_IT_number 96 _symmetry_cell_setting tetragonal _symmetry_space_group_name_Hall 'P 4nw 2abw' _symmetry_space_group_name_H-M 'P 43 21 2' _audit_creation_method SHELXL-97 _cell_angle_alpha 90.00 _cell_angle_beta 90.00 _cell_angle_gamma 90.00 _cell_formula_units_Z 4 _cell_length_a 10.3970(15) _cell_length_b 10.3970(15) _cell_length_c 29.262(6) _cell_measurement_reflns_used 32 _cell_measurement_temperature 212(2) _cell_measurement_theta_max 14.4 _cell_measurement_theta_min 11.2 _cell_volume 3163.2(9) _computing_cell_refinement STADI4 _computing_data_collection 'STADI4 (Stoe, 1998)' _computing_data_reduction 'X-RED (Stoe, 1998)' _computing_molecular_graphics 'local programs' _computing_publication_material 'local programs' _computing_structure_refinement 'SHELXL97 (Sheldrick, 1997)' _computing_structure_solution 'SHELXS97 (Sheldrick, 1990)' _diffrn_ambient_temperature 212(2) _diffrn_measured_fraction_theta_full 1.000 _diffrn_measured_fraction_theta_max 1.000 _diffrn_measurement_device_type 'Stoe Stadi-4' _diffrn_measurement_method \w _diffrn_radiation_monochromator graphite _diffrn_radiation_source 'fine-focus sealed tube' _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength .71073 _diffrn_reflns_av_R_equivalents .021 _diffrn_reflns_av_sigmaI/netI .0318 _diffrn_reflns_limit_h_max 12 _diffrn_reflns_limit_h_min 0 _diffrn_reflns_limit_k_max 12 _diffrn_reflns_limit_k_min 0 _diffrn_reflns_limit_l_max 34 _diffrn_reflns_limit_l_min 0 _diffrn_reflns_number 3161 _diffrn_reflns_theta_full 25.00 _diffrn_reflns_theta_max 25.00 _diffrn_reflns_theta_min 2.08 _diffrn_standards_decay_% 0 _diffrn_standards_interval_time 60 _diffrn_standards_number 3 _exptl_absorpt_coefficient_mu 1.486 _exptl_absorpt_correction_T_max .660 _exptl_absorpt_correction_T_min .596 _exptl_absorpt_correction_type empirical _exptl_absorpt_process_details 'X-RED (Stoe & Cie, 1998)' _exptl_crystal_colour orange _exptl_crystal_density_diffrn 1.513 _exptl_crystal_density_method 'not measured' _exptl_crystal_description octahedron _exptl_crystal_F_000 1472 _exptl_crystal_size_max .33 _exptl_crystal_size_mid .30 _exptl_crystal_size_min .28 _refine_diff_density_max .291 _refine_diff_density_min -.279 _refine_ls_abs_structure_details 'Flack (1983), 1094 Friedel pairs' _refine_ls_abs_structure_Flack -.06(3) _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.125 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 150 _refine_ls_number_reflns 2791 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.125 _refine_ls_R_factor_all .040 _refine_ls_R_factor_gt .029 _refine_ls_shift/su_max .001 _refine_ls_shift/su_mean .000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'calc w = 1/[\s^2^(Fo^2^)+(0.0079P)^2^+5.2275P] where P = (Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_ref .057 _reflns_number_gt 2527 _reflns_number_total 2791 _reflns_threshold_expression I>2\s(I) _cod_data_source_file qa0439.cif _cod_data_source_block I _cod_original_sg_symbol_Hall 'P 41n 2abw' _cod_database_code 2011644 loop_ _symmetry_equiv_pos_as_xyz 'x, y, z' '-x, -y, z+1/2' '-y+1/2, x+1/2, z+3/4' 'y+1/2, -x+1/2, z+1/4' '-x+1/2, y+1/2, -z+3/4' 'x+1/2, -y+1/2, -z+1/4' 'y, x, -z' '-y, -x, -z+1/2' loop_ _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_refinement_flags _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group _atom_site_type_symbol Te1 .43761(3) .56239(3) .7500 .02151(9) Uani d S 1 . . Te S11 .42914(12) .39940(10) .82649(4) .0287(3) Uani d . 1 . . S S12 .66612(11) .53125(12) .79778(4) .0339(3) Uani d . 1 . . S S21 .19313(11) .46936(11) .76072(4) .0329(3) Uani d . 1 . . S S22 .27112(11) .65413(13) .68924(4) .0336(3) Uani d . 1 . . S C1 .5912(4) .4240(4) .83389(13) .0269(10) Uani d . 1 . . C N1 .6578(4) .3632(4) .86666(13) .0351(10) Uani d . 1 . . N C11 .5945(6) .2774(5) .89921(17) .0474(15) Uani d . 1 . . C H11A .6457 .1987 .9021 .047 Uiso calc R 1 . . H H11B .5101 .2532 .8870 .047 Uiso calc R 1 . . H C12 .5765(7) .3350(6) .94570(19) .0697(19) Uani d . 1 . . C H12A .6597 .3468 .9601 .070 Uiso calc R 1 . . H H12B .5242 .2780 .9642 .070 Uiso calc R 1 . . H H12C .5338 .4176 .9429 .070 Uiso calc R 1 . . H C13 .7988(5) .3767(5) .87132(18) .0468(15) Uani d . 1 . . C H13A .8220 .3683 .9036 .047 Uiso calc R 1 . . H H13B .8239 .4631 .8613 .047 Uiso calc R 1 . . H C14 .8729(5) .2793(6) .8442(2) .0552(16) Uani d . 1 . . C H14A .8476 .1934 .8535 .055 Uiso calc R 1 . . H H14B .9642 .2908 .8495 .055 Uiso calc R 1 . . H H14C .8547 .2906 .8119 .055 Uiso calc R 1 . . H C2 .1502(4) .5677(5) .71586(14) .0277(10) Uani d . 1 . . C N2 .0285(3) .5801(4) .70322(12) .0330(10) Uani d . 1 . . N C21 -.0123(5) .6597(5) .66391(16) .0398(13) Uani d . 1 . . C H21A -.0754 .6119 .6457 .040 Uiso calc R 1 . . H H21B .0624 .6771 .6444 .040 Uiso calc R 1 . . H C22 -.0710(7) .7863(6) .67908(19) .0628(16) Uani d . 1 . . C H22A -.1558 .7708 .6917 .063 Uiso calc R 1 . . H H22B -.0781 .8436 .6530 .063 Uiso calc R 1 . . H H22C -.0167 .8254 .7022 .063 Uiso calc R 1 . . H C23 -.0755(5) .5178(5) .72878(16) .0379(12) Uani d . 1 . . C H23A -.1541 .5690 .7252 .038 Uiso calc R 1 . . H H23B -.0531 .5177 .7613 .038 Uiso calc R 1 . . H C24 -.1032(5) .3820(5) .71424(19) .0484(15) Uani d . 1 . . C H24A -.1259 .3808 .6821 .048 Uiso calc R 1 . . H H24B -.1742 .3482 .7321 .048 Uiso calc R 1 . . H H24C -.0275 .3293 .7191 .048 Uiso calc R 1 . . H loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Te1 .01978(11) .01978(11) .02498(18) -.00109(17) -.00064(13) -.00064(13) S11 .0280(6) .0259(6) .0324(6) -.0013(5) .0005(5) .0031(4) S12 .0259(6) .0408(8) .0349(6) -.0055(5) -.0031(5) .0047(6) S21 .0227(6) .0366(7) .0394(7) -.0056(5) -.0019(5) .0107(5) S22 .0223(6) .0440(7) .0346(7) -.0038(5) -.0011(5) .0122(6) C1 .031(3) .024(2) .0255(19) -.0011(19) -.0053(18) -.008(2) N1 .039(3) .034(2) .033(2) .0026(18) -.0145(19) .0010(19) C11 .055(4) .041(3) .046(3) .001(3) -.016(3) .016(3) C12 .077(5) .080(5) .052(4) -.003(4) .009(4) .009(3) C13 .039(3) .053(3) .048(3) .002(3) -.024(3) .002(3) C14 .036(3) .062(4) .068(4) .006(3) -.014(3) -.006(3) C2 .026(2) .032(2) .025(2) .001(2) -.0001(18) .000(2) N2 .021(2) .046(2) .032(2) -.0006(19) -.0015(16) .006(2) C21 .026(3) .063(4) .030(3) .000(3) -.006(2) .009(3) C22 .073(4) .063(4) .052(3) .008(4) .005(4) .015(3) C23 .018(2) .058(3) .037(3) -.009(2) .003(2) .002(2) C24 .038(3) .061(4) .047(3) -.009(3) .003(3) -.005(3) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C .0033 .0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H .0000 .0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N .0061 .0033 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' S S .1246 .1234 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Te Te -.5308 1.6751 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag S11 Te1 S11 8_666 . 132.28(5) yes S12 Te1 S11 8_666 8_666 63.58(3) no S12 Te1 S11 . 8_666 83.60(4) yes S12 Te1 S11 8_666 . 83.60(4) yes S12 Te1 S11 . . 63.58(3) yes S12 Te1 S12 8_666 . 93.10(5) yes S21 Te1 S11 . 8_666 131.50(3) yes S21 Te1 S11 8_666 8_666 70.51(3) no S21 Te1 S11 . . 70.51(3) yes S21 Te1 S11 8_666 . 131.50(3) yes S21 Te1 S12 . 8_666 82.16(4) yes S21 Te1 S12 8_666 8_666 134.09(3) no S21 Te1 S12 . . 134.09(3) yes S21 Te1 S12 8_666 . 82.16(4) yes S21 Te1 S21 . 8_666 132.01(5) yes S22 Te1 S11 . 8_666 81.30(4) yes S22 Te1 S11 8_666 8_666 136.80(4) no S22 Te1 S11 . . 136.80(4) yes S22 Te1 S11 8_666 . 81.30(4) yes S22 Te1 S12 . 8_666 92.64(4) yes S22 Te1 S12 8_666 8_666 159.41(4) no S22 Te1 S12 . . 159.41(4) yes S22 Te1 S12 8_666 . 92.64(4) yes S22 Te1 S21 . . 66.35(4) yes S22 Te1 S21 8_666 . 79.65(4) yes S22 Te1 S21 . 8_666 79.65(4) yes S22 Te1 S21 8_666 8_666 66.35(4) no S22 Te1 S22 . 8_666 88.86(6) yes C1 S11 Te1 . . 88.86(15) no C1 S12 Te1 . . 89.85(14) no C2 S21 Te1 . . 86.74(15) no C2 S22 Te1 . . 89.17(15) no S11 C1 S12 . . 117.5(2) no N1 C1 S11 . . 121.8(4) no N1 C1 S12 . . 120.7(4) no C1 N1 C11 . . 121.4(4) no C1 N1 C13 . . 122.2(4) no C11 N1 C13 . . 116.4(4) no N1 C11 C12 . . 113.8(5) no N1 C13 C14 . . 113.3(4) no S21 C2 S22 . . 117.6(2) no N2 C2 S21 . . 121.2(4) no N2 C2 S22 . . 121.2(4) no C2 N2 C21 . . 123.0(4) no C2 N2 C23 . . 121.3(4) no C23 N2 C21 . . 115.7(4) no N2 C21 C22 . . 111.9(4) no N2 C23 C24 . . 114.3(4) no loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag Te1 S11 8_666 2.8088(11) no Te1 S11 . 2.8088(11) yes Te1 S12 8_666 2.7758(12) no Te1 S12 . 2.7758(13) yes Te1 S21 . 2.7377(12) yes Te1 S21 8_666 2.7377(12) no Te1 S22 . 2.6584(13) yes Te1 S22 8_666 2.6584(13) no S11 C1 . 1.718(4) yes S12 C1 . 1.723(5) yes S21 C2 . 1.723(5) yes S22 C2 . 1.730(5) yes C1 N1 . 1.341(5) yes N1 C11 . 1.462(7) yes N1 C13 . 1.479(6) yes C11 C12 . 1.498(7) yes C13 C14 . 1.501(7) yes C2 N2 . 1.325(5) yes N2 C21 . 1.479(6) yes N2 C23 . 1.466(6) yes C21 C22 . 1.517(8) yes C23 C24 . 1.503(7) yes