#------------------------------------------------------------------------------ #$Date: 2026-09-03 22:12:44 +0100 (Thu, 03 Sep 2026) $ #$Revision: 306851 $ #$URL: svn://www.crystallography.net/cod/cif/2/02/35/2023550.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2023550 loop_ _publ_author_name 'Kumar, Sharatha' 'H\"okelek, Tuncer' _publ_section_title ; Synthesis, crystal structure determination, Hirshfeld surface and crystal void analyses, interaction energy calculations and energy frameworks of N-(2-methylphenyl)-N′-pivaloylthiourea ; _journal_coeditor_code WM5810 _journal_issue 10 _journal_name_full 'Acta Crystallographica Section E Crystallographic Communications' _journal_paper_doi 10.1107/S205698902600890X _journal_volume 82 _journal_year 2026 _chemical_formula_iupac 'C13 H18 N2 O S' _chemical_formula_moiety 'C13 H18 N2 O S' _chemical_formula_sum 'C13 H18 N2 O S' _chemical_formula_weight 250.35 _chemical_name_common ; N-(2-Methylphenyl)-N'-pivaloylthiourea ; _chemical_name_systematic ; 3-(2,2-Dimethylpropanoyl)-1-(2-methylphenyl)thiourea ; _space_group_crystal_system triclinic _space_group_IT_number 2 _space_group_name_Hall '-P 1' _space_group_name_H-M_alt 'P -1' _atom_sites_solution_hydrogens mixed _audit_creation_method SHELXL-2018/3 _cell_angle_alpha 63.290(4) _cell_angle_beta 81.600(3) _cell_angle_gamma 84.340(4) _cell_formula_units_Z 2 _cell_length_a 6.1050(4) _cell_length_b 10.7020(3) _cell_length_c 11.8910(3) _cell_measurement_reflns_used 2155 _cell_measurement_temperature 293(2) _cell_measurement_theta_max 27.71 _cell_measurement_theta_min 3.36 _cell_volume 686.08(6) _computing_cell_refinement ; CrysAlisRED (Oxford Diffraction, 2009) ; _computing_data_collection ; CrysAlisCCD (Oxford Diffraction, 2009) ; _computing_data_reduction ; CrysAlisRED (Oxford Diffraction, 2009) ; _computing_molecular_graphics ; Ortep-3 for Windows (Farrugia, 2012) ; _computing_publication_material ; WinGX (Farrugia, 2012) ; _computing_structure_refinement ; SHELXL (Sheldrick, 2015b) ; _computing_structure_solution ; SHELXT (Sheldrick, 2015a) ; _diffrn_ambient_temperature 293(2) _diffrn_measured_fraction_theta_full 0.990 _diffrn_measured_fraction_theta_max 0.981 _diffrn_measurement_device_type ; Oxford Diffraction Xcalibur with Sapphire CCD Detector ; _diffrn_measurement_method ; Rotation method data acquisition using omega scans. ; _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_av_R_equivalents 0.0103 _diffrn_reflns_av_unetI/netI 0.0152 _diffrn_reflns_limit_h_max 7 _diffrn_reflns_limit_h_min -7 _diffrn_reflns_limit_k_max 13 _diffrn_reflns_limit_k_min -13 _diffrn_reflns_limit_l_max 14 _diffrn_reflns_limit_l_min -10 _diffrn_reflns_number 4335 _diffrn_reflns_theta_full 25.242 _diffrn_reflns_theta_max 26.371 _diffrn_reflns_theta_min 3.376 _exptl_absorpt_coefficient_mu 0.223 _exptl_absorpt_correction_T_max 0.9652 _exptl_absorpt_correction_T_min 0.8967 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details ; (CrysAlis RED; Oxford Diffraction, 2009) ; _exptl_crystal_colour colourless _exptl_crystal_density_diffrn 1.212 _exptl_crystal_description prism _exptl_crystal_F_000 268 _exptl_crystal_size_max 0.500 _exptl_crystal_size_mid 0.480 _exptl_crystal_size_min 0.160 _refine_diff_density_max 0.713 _refine_diff_density_min -0.239 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.155 _refine_ls_hydrogen_treatment mixed _refine_ls_matrix_type full _refine_ls_number_parameters 160 _refine_ls_number_reflns 2756 _refine_ls_number_restraints 3 _refine_ls_restrained_S_all 1.156 _refine_ls_R_factor_all 0.0781 _refine_ls_R_factor_gt 0.0641 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0561P)^2^+0.6536P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1526 _refine_ls_wR_factor_ref 0.1639 _reflns_number_gt 2287 _reflns_number_total 2756 _reflns_threshold_expression 'I > 2\s(I)' _cod_data_source_file wm5810.cif _cod_data_source_block I _cod_database_code 2023550 _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _shelx_estimated_absorpt_t_min 0.897 _shelx_estimated_absorpt_t_max 0.965 _shelx_hkl_file ; 0 0 2 26677.8 90.3423 5 0 0 2 27139.6 92.7882 0 0 0 2 27065.5 98.8429 4 0 0 3 32015.6 125.411 0 0 0 3 32558.7 133.647 4 0 0 3 31913.7 121.159 5 0 0 4 19841.1 122.914 4 0 0 4 19591.4 115.630 0 0 0 5 46065.0 199.462 0 0 0 5 47449.4 213.273 4 0 0 6 87.2931 38.6731 4 0 0 7 869.862 54.0044 4 0 0 8 1595.78 71.2642 4 0 0 9 1395.77 76.2131 4 0 0 10 512.914 65.7899 4 0 0 11 3056.25 103.982 4 0 0 12 31.7530 64.2606 4 0 -1 11 11.9638 67.8520 4 0 -1 10 81.7986 60.7151 4 0 -1 9 710.622 68.1775 4 0 -1 8 5447.56 110.088 4 0 -1 7 3083.54 80.7887 4 0 -1 6 17400.1 154.035 4 0 -1 5 67107.9 225.246 2 0 -1 5 66789.4 125.780 6 0 -1 5 66103.0 266.214 4 0 -1 4 22932.1 122.270 1 0 -1 4 22693.7 76.3593 6 0 -1 4 23128.2 120.606 2 0 -1 4 22596.1 140.797 4 0 -1 3 2237.73 35.6613 2 0 -1 3 2286.17 38.0914 1 0 -1 3 2220.08 25.3518 6 0 -1 3 2082.25 44.7316 4 0 -1 2 119345. 191.872 5 0 -1 2 115887. 825.644 1 0 -1 2 118126. 235.170 4 0 -1 2 118383. 196.167 2 0 -1 1 48061.4 111.342 1 0 -1 1 48382.5 117.103 4 0 -1 1 48861.8 98.5419 2 0 1 2 15444.0 61.3946 3 0 1 2 15635.8 64.9203 4 0 1 2 15696.9 65.9272 0 0 1 2 15541.8 65.6513 5 0 1 3 5566.46 50.7137 0 0 1 3 5534.51 52.4875 4 0 1 4 16385.6 100.288 0 0 1 4 16464.1 103.002 4 0 1 5 41183.9 178.746 0 0 1 5 41193.5 185.675 4 0 1 6 8217.79 98.9570 4 0 1 6 8103.59 91.8349 0 0 1 7 257.037 34.9669 0 0 1 7 272.420 41.0072 4 0 1 8 346.336 47.8223 4 0 1 8 317.838 39.8321 0 0 1 9 9989.50 142.340 4 0 1 10 1762.70 78.6380 4 0 1 11 5895.52 129.728 4 0 1 12 3065.21 108.055 4 0 -2 12-23.7029 76.9805 4 0 -2 11 2552.10 108.039 4 0 -2 10 2004.89 90.9160 4 0 -2 9 330.494 58.1253 4 0 -2 8 1822.64 76.9261 4 0 -2 7 1524.47 68.3854 4 0 -2 7 1533.53 54.2606 2 0 -2 6 3260.86 65.3692 2 0 -2 6 2992.93 74.8657 4 0 -2 5 13136.5 112.451 1 0 -2 5 12621.7 126.971 4 0 -2 5 12991.5 107.229 2 0 -2 5 12543.0 76.5198 6 0 -2 4 58833.5 199.174 2 0 -2 4 58495.1 238.005 4 0 -2 4 58783.0 211.759 1 0 -2 4 57864.5 162.186 6 0 -2 3 4087.84 61.3898 4 0 -2 3 3898.80 53.2155 1 0 -2 3 3923.39 49.0702 2 0 -2 3 3752.14 42.1838 6 0 -2 2 129980. 230.432 2 0 -2 2 129976. 272.558 4 0 -2 2 130035. 229.361 6 0 -2 2 128596. 261.669 1 0 -2 1 76343.1 171.932 4 0 2 -1 76593.7 166.813 6 0 2 0-5.01397 16.6066 6 0 2 1 48580.3 123.917 6 0 2 2 227726. 1038.55 3 0 2 2 232870. 1021.62 6 0 2 3 55439.0 146.027 3 0 2 3 56344.3 151.138 0 0 2 3 56063.9 138.922 4 0 2 3 55623.1 124.198 6 0 2 4 7.21053 19.4884 4 0 2 4 7.37113 11.5723 6 0 2 4-1.98860 18.7675 3 0 2 4-3.35180 15.1672 0 0 2 5 5640.95 39.2144 6 0 2 5 5544.94 67.9189 4 0 2 5 5612.04 66.6119 0 0 2 6 2071.45 24.2163 6 0 2 6 2227.10 51.3352 0 0 2 6 2251.58 53.6494 4 0 2 7 94.4520 31.9121 0 0 2 7 115.455 34.9686 4 0 2 8 63.1101 36.7276 0 0 2 8 88.8821 42.4283 4 0 2 9 652.260 48.0601 0 0 2 9 674.553 56.5511 4 0 2 10 2018.69 78.9649 4 0 2 10 2188.00 79.0691 0 0 2 11 578.511 64.2310 0 0 2 11 310.150 60.1950 4 0 2 12 441.700 68.4804 4 0 2 13 289.145 72.6182 4 0 2 14 970.226 97.4876 4 0 -3 11 135.417 61.2511 4 0 -3 10 1454.67 85.5165 4 0 -3 9-9.30223 61.0772 4 0 -3 8 1831.51 64.4729 2 0 -3 8 1917.08 82.0389 4 0 -3 7 2486.33 84.8868 4 0 -3 7 2659.47 69.9706 2 0 -3 6 2891.13 78.3270 4 0 -3 6 2981.51 68.4957 1 0 -3 6 2962.25 64.5992 2 0 -3 5 34.7250 36.9804 4 0 -3 5 61.4106 29.7707 1 0 -3 5 52.8480 28.8540 2 0 -3 4 1076.13 32.6519 6 0 -3 4 1118.97 40.1996 1 0 -3 4 1061.36 44.0488 4 0 -3 4 1202.44 38.5311 2 0 -3 3 8256.32 88.8115 4 0 -3 3 8328.11 82.7326 1 0 -3 3 8246.72 74.2806 2 0 -3 3 8109.67 73.3473 6 0 -3 2 18934.9 113.686 1 0 -3 2 18756.0 99.8345 2 0 -3 2 18360.7 107.016 6 0 -3 2 18743.1 113.333 4 0 3 -1 230.957 22.6396 6 0 -3 1 253.778 20.0530 4 0 -3 0 3598.96 34.5631 4 0 3 0 3596.18 46.4527 6 0 3 1 173066. 291.167 6 0 3 2 35744.5 131.166 6 0 3 3 1229.63 21.3142 4 0 3 3 1206.52 28.6122 3 0 3 3 1254.41 29.8487 6 0 3 4 5652.07 56.9559 3 0 3 4 5672.43 52.6865 4 0 3 4 5447.29 50.7356 6 0 3 5 293.059 23.9862 3 0 3 5 267.502 24.8076 4 0 3 5 298.222 26.1703 0 0 3 5 282.829 18.9498 6 0 3 6 52.2279 27.6336 4 0 3 6 36.1810 14.6152 6 0 3 6 75.2701 25.6398 3 0 3 6 66.5874 27.8323 0 0 3 7 21753.2 152.245 0 0 3 7 22352.8 156.423 4 0 3 8 12951.6 133.895 4 0 3 8 12806.1 128.561 0 0 3 9 1316.65 59.6832 4 0 3 9 1403.25 56.7736 0 0 3 10 11697.8 145.308 0 0 3 10 11553.1 151.086 4 0 3 11-61.1374 52.6950 0 0 3 11 12.6175 53.8605 4 0 3 12 4815.67 114.103 0 0 3 12 5159.69 123.769 4 0 3 13 1345.68 87.7936 4 0 -4 10 345.558 67.9806 4 0 -4 9 619.330 70.5224 4 0 -4 8 162.832 55.2686 4 0 -4 8 317.560 45.8487 2 0 -4 7 2359.32 84.3814 4 0 -4 7 2490.40 71.7441 2 0 -4 6 1871.68 58.5123 2 0 -4 6 1835.65 62.1696 1 0 -4 6 1801.29 68.3732 4 0 -4 5 3571.97 80.9410 4 0 -4 5 3219.38 70.0228 1 0 -4 5 3428.67 66.5342 2 0 -4 4 9608.34 111.165 4 0 -4 4 9326.87 94.8350 2 0 -4 4 9554.02 90.0501 6 0 -4 4 9410.80 103.644 1 0 -4 3 7944.24 79.6036 2 0 -4 3 7748.19 82.4188 6 0 -4 3 7845.65 91.0225 4 0 -4 3 7670.79 88.3313 1 0 -4 2 54.6142 23.5967 4 0 -4 2 35.6304 23.1889 1 0 -4 2 47.3263 23.7408 6 0 -4 2 57.1662 20.6879 2 0 -4 1 12471.7 86.6286 4 0 4 -1 12500.4 96.9185 6 0 4 0 5897.20 68.0946 6 0 -4 0 5761.51 48.9771 4 0 4 1 193.548 27.8078 6 0 4 2 32450.1 146.692 6 0 4 3 11169.5 88.1256 6 0 4 4 3375.95 51.1164 6 0 4 4 3564.90 37.0749 4 0 4 4 3559.14 50.5913 3 0 4 5 7621.59 71.1005 6 0 4 5 7505.58 74.7722 3 0 4 5 7545.06 65.8301 4 0 4 6 5781.30 70.6702 3 0 4 6 5656.54 63.0155 6 0 4 6 5910.75 69.2147 4 0 4 6 5929.28 75.4792 0 0 4 7 1758.06 47.4876 3 0 4 7 1561.54 35.9511 6 0 4 7 1755.62 50.2341 4 0 4 7 1814.36 50.8348 0 0 4 8 643.434 42.6087 0 0 4 8 793.847 45.3012 4 0 4 9 1077.58 54.0260 4 0 4 9 1143.44 54.2168 0 0 4 10 6951.60 113.388 0 0 4 10 6744.82 114.326 4 0 4 11 4201.04 101.735 0 0 4 11 4167.46 101.250 4 0 4 12 12430.5 171.041 4 0 4 12 12750.7 170.657 0 0 4 13 1698.94 79.7941 0 0 4 13 1924.81 89.0700 4 0 4 14 154.454 67.8706 0 0 -5 10 393.219 79.9038 4 0 -5 9 582.227 76.7685 4 0 -5 8 103.328 56.7764 4 0 -5 7 7506.55 136.277 4 0 -5 7 7402.04 118.630 1 0 -5 7 7482.04 114.333 2 0 -5 6 3953.52 80.4664 2 0 -5 6 3782.76 85.0280 1 0 -5 6 3843.90 96.0573 4 0 -5 5 5780.57 89.7227 2 0 -5 5 5787.81 102.708 4 0 -5 5 5631.77 93.8279 1 0 -5 4 20338.3 159.800 1 0 -5 4 20158.5 146.238 2 0 -5 4 20224.8 166.686 4 0 -5 4 20090.3 145.540 6 0 -5 3 41560.9 205.862 6 0 -5 3 41922.9 215.949 4 0 -5 3 42243.2 216.984 1 0 -5 3 41695.2 192.625 2 0 -5 2 2369.91 52.9265 4 0 -5 2 2300.00 55.1826 6 0 -5 2 2416.38 54.8274 1 0 -5 1 11706.4 108.106 6 0 5 -1 11939.8 106.663 6 0 -5 1 11805.4 92.3474 4 0 -5 0 10327.3 72.3248 4 0 5 0 10417.5 98.8843 6 0 5 1 36761.1 178.626 6 0 5 2 2463.49 54.4746 6 0 5 3 1590.64 44.8403 6 0 5 4 12113.8 103.696 6 0 5 5 9.51874 24.6160 6 0 5 5 42.5662 14.9768 4 0 5 5 8.49631 23.5451 3 0 5 6 26676.2 146.135 6 0 5 6 26874.9 132.257 4 0 5 6 26690.9 149.215 3 0 5 7 40133.5 202.924 0 0 5 7 40058.0 185.410 4 0 5 7 39927.2 191.843 3 0 5 7 40418.5 177.020 6 0 5 8 5915.44 84.6268 4 0 5 8 5940.23 89.1915 0 0 5 8 5828.14 83.6981 3 0 5 9 9.29374 32.9645 4 0 5 9-0.93719 37.3225 0 0 5 10 894.943 55.6734 0 0 5 10 828.968 52.6862 4 0 5 11 2286.48 80.4331 0 0 5 11 2236.85 76.6843 4 0 5 12 4775.17 109.357 0 0 5 12 5079.45 112.746 4 0 5 13 74.1806 50.5620 0 0 5 13 286.009 61.6566 4 0 5 14 64.0194 57.0167 4 0 -6 9 1576.64 101.039 4 0 -6 8 2485.72 99.3248 4 0 -6 7 108.189 55.7608 4 0 -6 7-1.99068 45.3581 1 0 -6 6 2328.52 74.7778 1 0 -6 6 2394.38 86.1271 4 0 -6 6 2271.51 67.8013 2 0 -6 5 6479.53 98.4744 2 0 -6 5 6473.00 113.435 4 0 -6 5 6461.10 106.097 1 0 -6 4 1092.60 57.4590 4 0 -6 4 992.415 48.0755 2 0 -6 4 1052.70 54.1447 1 0 -6 3 582.090 41.1354 6 0 -6 3 494.572 37.7258 2 0 -6 3 640.564 45.3506 4 0 -6 3 552.553 43.3553 1 0 -6 2 2781.19 64.8269 1 0 -6 2 2988.89 61.4905 4 0 -6 2 2745.37 64.7807 6 0 -6 1 17799.1 119.607 4 0 -6 1 17886.7 147.729 6 0 -6 0 7413.63 66.3208 4 0 6 0 7553.13 94.7509 6 0 6 1 18705.9 143.323 6 0 6 2 32633.7 186.089 6 0 6 3 12102.1 115.383 6 0 6 4 4500.37 74.1893 6 0 6 5 17684.4 135.874 6 0 6 5 17894.5 124.303 3 0 6 6 1585.22 49.5065 6 0 6 6 1689.32 48.4903 3 0 6 7 57.1666 30.2659 6 0 6 7 108.385 32.1546 0 0 6 7 64.4185 30.6798 3 0 6 8 8396.37 94.0680 6 0 6 8 8166.82 99.4502 3 0 6 8 8388.61 105.344 0 0 6 9 232.121 38.6345 3 0 6 9 231.849 40.7131 0 0 6 10 5.44300 36.6310 0 0 6 11 1923.05 72.1350 0 0 6 12 103.608 58.0313 0 0 6 13 4474.48 109.670 0 0 6 14 888.903 66.1842 0 0 -7 7 510.122 57.3805 1 0 -7 6 939.720 60.4384 1 0 -7 5 126.415 36.4578 1 0 -7 5 154.832 40.8075 2 0 -7 4 10959.8 135.348 1 0 -7 4 10979.7 123.622 2 0 -7 3 20068.7 173.546 6 0 -7 3 19474.1 154.018 2 0 -7 3 19722.4 171.019 1 0 -7 2 1848.17 62.5446 6 0 -7 2 1761.50 54.0546 2 0 -7 2 1710.80 59.9919 1 0 -7 1 9.80930 35.3759 6 0 -7 1-8.49047 30.8746 1 0 -7 0 4961.96 89.1660 6 0 7 1 3882.12 78.6407 6 0 7 2 21.3576 32.2414 6 0 7 3 1165.45 53.1290 6 0 7 4 226.067 41.6250 6 0 7 5 4648.17 82.7548 6 0 7 6 3146.27 63.1697 3 0 7 6 3155.91 69.2803 6 0 7 7 36.6753 34.8834 6 0 7 7 47.6812 29.1156 3 0 7 8 9466.49 114.051 0 0 7 8 9570.80 109.842 3 0 7 8 9331.89 109.482 6 0 7 9 389.880 44.3755 0 0 7 9 250.361 39.7801 3 0 7 10 2506.07 68.0402 3 0 7 10 2548.56 75.0984 0 0 7 11 2672.78 78.5359 0 0 7 12-40.6603 47.7923 0 0 7 13 188.368 56.4165 0 0 -8 6 894.003 65.7307 1 0 -8 5 346.473 54.5610 1 0 -8 4 297.123 48.4270 1 0 -8 3 1363.67 62.4441 1 0 -8 3 1184.92 53.9080 2 0 -8 2 6.64275 39.3415 2 0 -8 2 15.1152 39.8603 1 0 -8 2 66.3287 43.0368 6 0 -8 1 3290.78 84.9047 6 0 -8 1 3410.72 76.6334 1 0 -8 0 5834.39 103.235 6 0 -8 -1 3953.57 87.3636 6 0 8 2 2184.03 68.8287 6 0 8 3 5492.44 96.8169 6 0 8 4 1160.82 55.9329 6 0 8 5 18.0935 38.1885 6 0 8 6 2504.14 60.9569 3 0 8 6 2489.24 72.1925 6 0 8 7 1280.35 52.9329 3 0 8 7 1369.90 60.1680 6 0 8 8 6024.86 98.7325 6 0 8 8 6114.56 94.8915 3 0 8 9 1905.54 61.2710 3 0 8 9 1882.80 63.6766 0 0 8 9 1972.84 62.3040 6 0 8 10 70.3073 39.5776 3 0 8 10 107.429 40.8331 0 0 8 11 877.794 53.0337 3 0 8 11 914.057 57.1046 0 0 8 12 882.114 61.6262 0 0 8 13 281.792 46.0568 0 0 8 14 315.538 62.5111 0 0 -9 5 3467.95 100.091 1 0 -9 4 2402.78 80.0345 1 0 -9 3 73.9951 44.5431 1 0 -9 2 243.920 38.3169 2 0 -9 2 144.278 45.3495 6 0 -9 2 142.628 45.4714 1 0 -9 1 32.1187 40.0342 1 0 -9 1 93.1833 51.6375 6 0 -9 0 109.984 48.5725 6 0 -9 -1 42.0887 46.6393 6 0 -9 -2 295.010 54.7163 6 0 9 3 331.328 49.6179 6 0 9 4 62.2677 45.6196 6 0 9 5 6822.61 115.303 6 0 9 6 7195.24 117.299 6 0 9 7 1187.62 54.8738 3 0 9 7 994.727 58.7005 6 0 9 8 4083.12 81.8655 3 0 9 8 4103.83 91.0921 6 0 9 9 5698.83 103.703 6 0 9 9 5921.60 99.1616 3 0 9 10 67.7706 37.1289 3 0 9 10 8.55366 40.7725 0 0 9 11 56.8199 42.0018 3 0 9 11 7.42999 39.9716 0 0 9 12 901.274 56.6661 3 0 9 12 984.626 63.6994 0 0 9 13 922.792 57.1999 0 0 9 14 231.430 57.2004 0 0 -10 4-23.4152 44.0760 1 0 -10 3 1218.83 67.6611 1 0 -10 2 303.537 49.8581 1 0 -10 2 175.762 57.2276 6 0 -10 1 1111.39 58.1835 1 0 -10 1 1071.49 66.0997 6 0 -10 0 5952.07 106.451 1 0 -10 0 5820.43 119.869 6 0 -10 -1 379.289 59.4937 6 0 -10 -2 69.0752 51.8190 6 0 -10 -3 3570.75 99.6648 6 0 10 4 7660.23 130.522 6 0 10 5 5535.60 113.234 6 0 10 6 2670.05 88.1307 6 0 10 7 4576.33 101.528 6 0 10 7 5015.15 93.0205 3 0 10 8 2395.76 81.4391 6 0 10 8 2574.44 73.6122 3 0 10 9 3479.89 84.0957 3 0 10 9 3250.78 91.2314 6 0 10 10 20.6118 37.1522 3 0 10 10-9.42299 41.9608 0 0 10 11 803.984 56.7863 0 0 10 11 721.198 54.9962 3 0 10 12 2.79763 41.5152 0 0 10 12 178.025 46.9273 3 0 10 13 324.875 54.3245 0 0 10 13-41.0368 45.6152 3 0 -11 2 851.895 66.6244 1 0 -11 1 524.687 57.6984 1 0 -11 1 640.232 69.5575 6 0 -11 0 219.726 45.7541 1 0 -11 0 111.398 61.9710 6 0 -11 -1 3820.43 91.0173 1 0 -11 -1 4272.53 110.300 6 0 -11 -2 2883.88 98.2652 6 0 -11 -3 30.3134 50.0523 6 0 -11 -4 2032.82 88.6107 6 0 -11 -5 417.647 60.8211 6 0 11 6 118.355 50.5236 6 0 -11 -6 88.5469 56.2995 6 0 11 7 61.4858 54.3443 6 0 11 8 1368.51 75.4945 6 0 11 9 3090.93 96.6679 6 0 -11 -10 680.705 59.5260 6 0 11 11-10.4981 39.7951 0 0 11 12 783.144 58.6724 0 0 11 13 7.22555 46.6105 0 0 -12 1 357.063 61.1695 6 0 -12 1 41.8288 48.1066 1 0 -12 -1 220.275 72.9091 6 0 -12 -2 338.610 72.9593 6 0 -12 -3 3758.03 118.482 6 0 -12 -4 1724.51 83.5655 6 0 -12 -5 270.245 67.5806 6 0 -12 -6 515.585 69.2342 6 0 -12 -7 1174.75 75.3279 6 0 -12 -8 1378.65 75.5740 6 0 -12 -9 264.434 57.7139 6 0 -12 -10 247.152 61.3739 6 0 12 12 182.726 52.2490 0 0 -13 -4 211.874 74.1520 6 0 -13 -5 323.550 61.8916 6 0 -13 -7 743.973 79.6706 6 0 -13 -8 385.299 66.1213 6 1 -13 -10 27.7902 63.0103 6 1 -13 -9-61.2216 52.5808 6 1 -13 -8 56.2676 61.4642 6 1 -13 -7 405.208 65.1233 6 1 -13 -6 52.0307 64.0124 6 -1 12 12 254.653 50.2484 3 -1 12 10 1073.74 70.6364 3 1 -12 -9 254.343 59.8012 6 -1 12 9 350.778 56.0729 3 1 -12 -8-10.2353 50.8596 6 -1 12 8 41.3568 44.6228 3 1 -12 -7 268.615 54.8470 6 1 -12 -6 3056.82 106.413 6 1 -12 -5 794.923 69.4579 6 1 -12 -4-63.4714 52.2373 6 1 -12 -3 880.569 81.5089 6 1 -12 -2 692.317 75.0515 6 1 -12 -1 238.199 60.1093 6 1 -12 0 494.293 64.6923 1 1 -12 0 442.880 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62.4417 1 -1 8 14 958.844 66.0719 0 -1 8 13 775.112 60.3146 0 -1 8 12 1200.93 63.7567 3 -1 8 12 1164.95 63.2339 0 -1 8 11 2011.10 73.7930 3 -1 8 11 1938.42 72.1595 0 -1 8 10 118.042 39.6291 3 -1 8 10 67.4351 35.3661 0 -1 8 9 910.617 55.5762 3 -1 8 9 1064.80 53.8325 0 -1 8 8 189.722 35.2628 0 -1 8 8 190.783 41.6884 3 1 -8 -8 282.478 41.5986 6 -1 8 7 8512.62 116.281 3 1 -8 -7 8027.23 113.915 6 1 -8 -6 9740.67 128.189 6 1 -8 -5 2534.94 76.1562 6 1 -8 -4 9175.12 125.067 6 1 -8 -3 6597.19 110.309 6 1 -8 -2 44.3439 43.7631 6 1 -8 -1-6.76200 43.3243 6 1 -8 0 6190.50 109.565 6 1 -8 1 869.008 59.8266 6 1 -8 2 1181.69 63.8450 6 1 -8 3 15.8215 42.9438 6 1 -8 3 93.0505 45.1112 1 1 -8 4 715.752 58.9654 1 1 -8 5 139.769 43.2468 1 1 -8 6 3428.39 94.3425 1 -1 7 14 709.264 61.0404 0 -1 7 13 628.371 53.3621 0 -1 7 12 500.188 55.6837 0 -1 7 11 899.181 53.8862 3 -1 7 11 971.728 55.4575 0 -1 7 10 962.191 54.8207 3 -1 7 10 893.365 49.2577 0 -1 7 9 3257.47 76.3122 0 -1 7 9 3121.09 76.9481 3 -1 7 8 1217.89 53.2166 3 1 -7 -8 1389.62 50.8688 6 -1 7 8 1418.83 53.0364 0 1 -7 -7 9615.18 111.937 6 -1 7 7 9632.23 108.783 0 -1 7 7 9744.08 117.988 3 1 -7 -6 19973.1 161.524 6 -1 7 6 20528.3 160.612 3 1 -7 -5 5264.36 89.7771 6 1 -7 -4 914.008 52.9995 6 1 -7 -3 9987.15 121.918 6 1 -7 -2 11763.8 131.995 6 1 -7 -1 113.430 41.0371 6 1 -7 0 1394.49 56.4899 6 1 -7 1 132.997 37.9667 6 1 -7 2 9428.15 124.838 6 1 -7 3 2939.48 79.6405 6 1 -7 3 2820.57 74.9955 1 1 -7 4 408.426 45.2849 1 1 -7 5 121.700 43.5811 1 1 -7 6 73.1302 42.0796 1 1 -7 7 581.796 58.2074 1 -1 6 13 247.395 58.4556 0 -1 6 12 815.519 64.4348 0 -1 6 11 4315.32 97.7506 0 -1 6 10 407.202 48.4798 3 -1 6 10 362.128 46.2734 0 -1 6 9 4841.38 87.6122 0 -1 6 9 4666.15 87.9909 3 -1 6 8 11121.4 123.688 3 -1 6 8 10780.8 118.112 0 -1 6 7 1365.03 46.6064 0 -1 6 7 1278.57 51.6561 3 1 -6 -7 1471.36 47.5025 6 1 -6 -6 3998.87 70.4060 6 -1 6 6 4162.95 64.4890 5 -1 6 6 4314.69 76.2585 3 -1 6 5 1414.80 37.1238 5 1 -6 -5 1399.42 48.0556 6 -1 6 4 1940.67 35.8085 5 1 -6 -4 1901.72 55.0014 6 1 -6 -3 37135.6 205.326 6 1 -6 -2 1596.85 55.6749 6 1 -6 -1 44.7862 33.6802 6 1 -6 0 216.623 38.0279 6 1 -6 1 16238.4 145.593 6 1 -6 2 844.165 46.4462 6 1 -6 3 2186.53 63.9126 6 1 -6 3 2047.03 64.7851 1 1 -6 4 4274.33 87.9152 1 1 -6 4 4665.02 86.4438 6 1 -6 5 11268.2 137.824 1 1 -6 6 1974.33 72.9208 1 1 -6 7 1398.13 66.8265 1 1 -6 8 513.411 55.3108 1 -1 5 14 819.920 75.5585 0 -1 5 13 547.725 59.0365 0 -1 5 12 4452.53 110.424 0 -1 5 12 4771.05 113.379 4 -1 5 11 2401.44 79.2359 4 -1 5 11 2307.86 80.3055 0 -1 5 10 5396.63 102.659 0 -1 5 10 5913.91 104.591 4 -1 5 9 59.4760 37.2679 4 -1 5 9 46.8381 34.6474 3 -1 5 9 6.97484 38.5708 0 -1 5 8 387.622 37.3843 4 -1 5 8 369.924 38.4423 3 -1 5 8 348.215 35.9769 0 -1 5 7 1173.07 40.3809 4 1 -5 -7 1247.88 39.3689 6 -1 5 7 1103.64 46.8894 5 -1 5 7 1072.39 46.9139 3 -1 5 7 1129.61 42.4320 0 1 -5 -6 593.886 32.7645 6 -1 5 6 556.521 27.1332 4 -1 5 6 564.628 33.0260 0 -1 5 6 594.891 39.5670 3 -1 5 6 549.470 35.0625 5 -1 5 5 1950.33 45.1602 5 1 -5 -5 1859.52 47.3340 6 -1 5 5 1976.14 51.3174 3 1 -5 -4 66087.5 241.339 6 -1 5 4 65527.1 194.701 5 -1 5 3 3860.24 43.0005 5 1 -5 -3 3854.32 65.9482 6 -1 5 2 1191.24 20.8594 5 1 -5 -2 1257.83 45.3810 6 1 -5 -1 15.4585 29.9232 6 1 -5 -1 38.7949 9.47001 4 1 -5 0 3680.60 43.6627 4 1 -5 0 3589.22 66.2193 6 1 -5 1 43941.9 170.561 4 1 -5 1 44880.4 217.211 6 1 -5 2 509.642 32.0222 4 1 -5 2 468.659 38.9869 6 1 -5 3 2450.10 58.6224 4 1 -5 3 2314.49 60.7780 1 1 -5 3 2402.73 46.9708 2 1 -5 3 2308.92 61.1973 6 1 -5 4 61.9516 36.0206 4 1 -5 4 31.8883 35.2898 1 1 -5 4-2.87354 24.3482 2 1 -5 4 80.3644 33.4484 6 1 -5 5 353.469 46.9259 4 1 -5 5 303.649 47.4422 1 1 -5 6 404.632 46.8689 1 1 -5 6 362.387 52.4965 4 1 -5 7 4104.74 92.0953 1 1 -5 7 4170.60 105.481 4 1 -5 8 2733.00 98.8972 4 1 -5 8 2515.99 80.7238 1 1 -5 9 227.598 73.2652 4 1 -5 10 2964.80 119.665 4 -1 4 14 213.933 75.2903 4 -1 4 13 253.917 55.5049 0 -1 4 13 373.013 60.8855 4 -1 4 12 1173.37 70.3094 0 -1 4 12 1518.21 79.0887 4 -1 4 11 2745.39 87.0907 0 -1 4 11 3003.18 90.6783 4 -1 4 10 11910.5 147.638 4 -1 4 10 12093.8 148.452 0 -1 4 9 6857.38 104.114 0 -1 4 9 6783.45 104.992 4 -1 4 8 4261.09 78.6885 4 -1 4 8 4067.08 79.6233 5 -1 4 8 4421.85 78.9835 0 -1 4 8 4212.87 76.3960 3 -1 4 7 14.5278 27.3660 0 -1 4 7 34.8193 27.3721 4 -1 4 7 62.6747 27.4554 3 -1 4 7 92.0856 35.1580 5 -1 4 6 39837.8 193.762 5 -1 4 6 39842.4 175.558 4 1 -4 -6 39236.1 158.368 6 -1 4 6 39480.8 194.257 3 -1 4 6 40102.7 185.081 0 -1 4 5 54538.9 218.592 3 1 -4 -5 55651.1 192.690 6 -1 4 5 55493.8 198.009 0 -1 4 5 56115.0 207.537 5 -1 4 5 55391.6 176.197 4 -1 4 4 48392.0 173.119 5 1 -4 -4 48433.4 183.591 6 1 -4 -3 14862.4 106.227 6 -1 4 3 15066.3 86.3339 5 1 -4 -2 5939.07 70.2949 6 -1 4 2 5959.69 45.7578 5 1 -4 -1 14005.6 107.394 6 1 -4 0 2986.66 36.5311 4 1 -4 0 2923.77 56.8625 6 1 -4 1 33126.3 170.646 6 1 -4 1 33238.1 138.351 4 1 -4 2 11114.4 102.888 6 1 -4 2 11123.0 76.4548 2 1 -4 2 10968.4 93.7184 4 1 -4 3 4835.52 72.4976 6 1 -4 3 4933.66 57.5532 2 1 -4 3 4923.61 73.0460 4 1 -4 4 2186.67 58.0706 1 1 -4 4 2178.34 59.7126 4 1 -4 4 2250.02 46.3084 2 1 -4 4 2197.03 53.1384 6 1 -4 5 20188.5 140.742 6 1 -4 5 20633.2 163.686 1 1 -4 5 20429.6 174.649 4 1 -4 5 20534.3 135.522 2 1 -4 6 27945.9 197.503 1 1 -4 6 27781.4 218.417 4 1 -4 7 340.468 42.3382 1 1 -4 7 187.418 54.5477 4 1 -4 8 2219.78 74.6338 1 1 -4 8 2136.14 89.8063 4 1 -4 9 516.795 66.7613 4 1 -4 10 1004.21 82.7200 4 -1 3 14 448.392 83.5421 4 -1 3 13 571.605 68.3088 4 -1 3 12 228.308 67.7263 4 -1 3 11 4135.60 110.206 4 -1 3 11 3983.11 100.429 0 -1 3 10 15398.2 167.409 0 -1 3 10 16212.6 178.304 4 -1 3 9 1926.83 69.0114 4 -1 3 9 2157.15 69.1529 0 -1 3 8 844.085 51.3924 5 -1 3 8 950.506 48.4138 0 -1 3 8 870.441 49.8579 4 -1 3 7 5617.84 86.6970 5 -1 3 7 5714.31 81.6513 0 -1 3 7 5862.95 85.2586 4 -1 3 7 5626.42 79.8500 3 1 -3 -6 873.523 24.2416 6 -1 3 6 932.632 37.2042 0 -1 3 6 801.593 40.4054 3 -1 3 6 920.091 44.7060 5 -1 3 6 941.004 40.0039 4 1 -3 -5 1042.71 27.5872 6 -1 3 5 1012.96 39.2623 3 -1 3 5 1053.06 40.8130 5 -1 3 5 1029.69 33.7496 0 -1 3 5 1128.17 35.4368 4 1 -3 -4 1395.44 31.7185 6 -1 3 4 1413.97 31.7656 4 -1 3 4 1490.26 33.5476 0 -1 3 4 1548.24 39.6598 5 -1 3 4 1512.13 40.8256 3 -1 3 3 46452.9 152.287 5 1 -3 -3 47182.9 160.382 6 1 -3 -2 185591. 323.164 6 -1 3 2 186021. 1038.77 5 -1 3 1 320679. 1138.43 5 1 -3 -1 322524. 1749.24 6 1 -3 0 35390.1 106.254 4 1 -3 0 35275.2 151.502 6 1 -3 1 12046.4 93.3472 6 1 -3 1 12234.7 77.7341 4 1 -3 2 3840.72 53.9316 4 1 -3 2 3826.51 56.7381 6 1 -3 2 3963.71 41.1006 2 1 -3 3 10318.7 73.0739 2 1 -3 3 9776.94 94.1812 4 1 -3 3 10201.7 89.7059 6 1 -3 4 26597.8 142.736 6 1 -3 4 25770.8 166.642 4 1 -3 4 26377.1 161.468 1 1 -3 4 26484.0 130.184 2 1 -3 5 1947.85 60.9672 4 1 -3 5 2011.27 44.0588 6 1 -3 5 2008.43 45.0920 2 1 -3 5 1994.89 54.4861 1 1 -3 6 10868.9 107.013 2 1 -3 6 10304.6 130.505 4 1 -3 6 10573.5 117.445 1 1 -3 7 10492.5 124.262 1 1 -3 7 10579.1 146.321 4 1 -3 8-25.9711 54.0219 4 1 -3 8-31.0795 42.4029 1 1 -3 9-20.9516 61.3024 4 1 -3 10 512.006 64.8391 4 1 -3 11 200.747 77.5052 4 -1 2 13 982.853 85.7349 4 -1 2 12 111.730 62.6557 4 -1 2 11 3600.34 106.347 4 -1 2 10 7480.22 132.496 4 -1 2 9 16902.6 167.101 0 -1 2 9 16448.7 173.199 4 -1 2 8 3750.75 77.5290 0 -1 2 8 3292.43 79.1785 5 -1 2 8 3625.57 82.1624 4 -1 2 7-24.1782 34.5006 4 -1 2 7 8.31318 27.5229 0 -1 2 7 34.9954 38.0111 5 -1 2 6 36968.2 193.830 5 -1 2 6 37241.7 194.698 4 -1 2 6 37523.2 189.541 0 -1 2 6 37743.6 179.455 3 -1 2 5 28849.4 153.790 4 -1 2 5 29082.2 145.932 3 -1 2 5 28512.1 156.532 5 1 -2 -5 29003.9 90.5879 6 -1 2 5 29072.1 146.949 0 1 -2 -4 44807.6 121.584 6 -1 2 4 44572.3 176.863 5 -1 2 4 44961.8 165.355 4 -1 2 4 45401.7 168.460 3 -1 2 4 44910.1 159.837 0 1 -2 -3 12501.3 69.1025 6 -1 2 3 12899.9 86.2716 3 -1 2 3 11878.7 80.1270 5 -1 2 3 12217.0 73.6419 4 -1 2 3 12057.6 71.6333 0 -1 2 2 38870.1 124.918 5 1 -2 -2 39292.5 126.743 6 -1 2 2 39070.2 104.051 0 1 -2 -1 193525. 1165.77 6 1 -2 0 5650.89 54.2402 6 1 -2 1 41542.7 146.642 6 1 -2 2 36511.1 143.077 6 1 -2 2 37033.7 99.3499 2 1 -2 2 36299.9 145.413 4 1 -2 3 1439.52 33.6575 6 1 -2 3 1517.71 28.1940 2 1 -2 3 1368.65 39.7710 4 1 -2 4 5863.36 59.1387 2 1 -2 4 5495.50 76.7343 4 1 -2 4 5585.26 58.7945 6 1 -2 4 5725.61 71.4684 1 1 -2 5 1215.57 31.2803 6 1 -2 5 1258.71 41.9618 1 1 -2 5 1188.61 47.6162 4 1 -2 5 1241.40 37.4519 2 1 -2 6 977.903 54.0721 4 1 -2 6 945.142 42.9154 1 1 -2 7 7416.25 99.5472 1 1 -2 7 7326.27 116.430 4 1 -2 8 1792.19 79.8693 4 1 -2 9 7033.32 135.605 4 1 -2 10 515.681 64.6014 4 1 -2 11 481.452 76.1245 4 1 -2 12 133.578 73.9414 4 -1 1 13 233.703 63.6937 4 -1 1 12 1483.15 91.5076 4 -1 1 11 617.638 65.3807 4 -1 1 10 2098.00 83.7790 4 -1 1 9 1250.35 68.5066 4 -1 1 8 1686.70 67.7802 4 -1 1 8 1699.92 63.5523 5 -1 1 7 218.412 39.5189 5 -1 1 7 121.657 37.1422 4 -1 1 6 3400.28 64.3196 0 -1 1 6 3322.07 69.4880 4 -1 1 6 3322.89 67.8305 5 -1 1 5 12905.5 111.799 4 -1 1 5 13229.3 106.488 0 -1 1 5 13101.2 110.473 5 -1 1 4 17037.9 100.416 3 -1 1 4 17044.3 112.936 5 -1 1 4 17369.1 113.219 4 -1 1 4 17185.4 105.051 0 -1 1 3 2651.17 43.4505 4 -1 1 3 2667.34 44.3985 5 -1 1 3 2835.85 40.5027 3 -1 1 3 2795.18 39.1776 0 -1 1 2 252421. 1079.86 0 -1 1 2 252952. 1295.17 5 1 -1 -2 252222. 957.580 6 1 -1 -1 486.622 16.9839 6 1 -1 0 173027. 921.101 6 1 -1 1 34565.3 108.939 6 1 -1 2 74103.0 165.482 6 1 -1 2 74235.5 190.294 4 1 -1 3 7434.00 73.4242 4 1 -1 3 7548.34 56.6512 6 1 -1 3 7531.92 65.0875 1 1 -1 3 7641.81 51.0089 2 1 -1 4 1054.91 38.1100 4 1 -1 4 1219.72 35.2618 1 1 -1 4 1141.30 26.3849 6 1 -1 5 356.182 37.9310 4 1 -1 5 276.592 17.5516 6 1 -1 5 318.313 26.9862 1 1 -1 6 7591.78 85.7924 1 1 -1 6 7107.07 100.736 4 1 -1 6 7285.15 58.4204 6 1 -1 7 2579.95 58.9018 1 1 -1 7 2395.44 72.5592 4 1 -1 8 593.286 60.2615 4 1 -1 9 690.194 66.7785 4 1 -1 10 1128.77 77.4975 4 1 -1 11-90.9005 54.4477 4 1 -1 12 54.3862 71.6922 4 -1 0 12 499.914 82.9725 4 -1 0 11 1543.14 83.2235 4 -1 0 10 6567.99 130.685 4 -1 0 9 3435.23 96.5016 4 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69.4321 6 6 6 2 1206.00 69.1408 6 6 6 3-19.3930 47.9508 6 6 6 4 574.257 60.5433 6 6 6 5 216.938 55.6303 6 6 6 6 329.651 59.3596 6 6 6 7 109.255 53.2194 6 6 6 8 139.688 54.3024 6 6 6 9 306.640 61.6405 6 6 6 10 334.693 64.8934 6 6 6 11 219.766 65.4502 6 -6 -7 1 284.021 55.0075 2 -6 -7 0 758.082 59.1850 2 6 7 1-109.019 55.4137 6 -6 -7 -1-58.4081 44.5419 2 6 7 2 144.981 52.6101 6 -6 -7 -2 83.7419 45.7124 2 6 7 3 95.5221 54.8357 6 6 7 4 19.7422 51.9085 6 6 7 5-46.5286 44.8796 6 6 7 6-36.7874 44.8562 6 6 7 7 129.097 57.9917 6 6 7 8-14.1628 55.1638 6 6 7 9-78.3736 58.8406 6 6 7 10 23.7641 48.1373 6 6 7 11 192.044 58.6307 6 -6 -8 0 720.175 69.7414 2 -6 -8 -1 162.943 57.4697 2 6 8 1 701.639 73.5450 6 6 8 2 87.1910 56.2216 6 -6 -8 -2 207.871 54.3232 2 6 8 3-113.833 58.9964 6 -6 -8 -3 77.7425 49.1497 2 6 8 4-15.5665 52.2691 6 6 8 5 211.000 64.5823 6 6 8 6 128.922 69.6556 6 6 8 7 546.036 71.3531 6 6 8 8 210.869 70.6972 6 6 8 9 172.360 70.0151 6 6 8 10 233.659 71.3579 6 6 9 2-109.713 70.7136 6 -6 -9 -2 178.790 58.5741 2 6 9 3 237.784 73.8421 6 -6 -9 -3 140.808 49.6200 2 6 9 4 234.503 73.3502 6 6 9 5-35.0377 55.3620 6 6 9 6-71.5412 68.4520 6 6 9 7-92.1477 59.1520 6 7 -5 -3 402.818 45.4296 6 -7 4 4 234.949 83.1599 5 7 -4 -3-88.7225 39.3478 6 7 -4 -2 1124.41 55.5045 6 -7 4 2 1163.78 82.1124 5 7 -4 -1 1755.00 71.3214 6 7 -4 0 1437.48 70.2390 6 -7 3 4 1195.14 98.6806 5 -7 3 3 685.138 83.3785 5 -7 3 2 125.548 65.2667 5 7 -3 -1 160.859 32.6480 6 -7 3 1 175.692 72.3072 5 7 -3 0-12.6936 39.0680 6 7 -3 1 374.662 45.4310 6 7 -3 2-44.8466 39.7993 6 -7 2 4 10.2677 71.4932 5 -7 2 3 891.218 80.8285 5 7 -2 -2 1800.19 62.3239 6 -7 2 2 1606.85 98.9039 5 7 -2 -1 759.497 50.5678 6 7 -2 0 147.483 41.7516 6 7 -2 1 196.361 45.4503 6 7 -2 2-6.02579 43.9559 6 7 -2 3 374.102 54.2929 6 7 -2 4 357.400 50.8523 6 -7 1 3-71.1684 66.4324 5 -7 1 2 58.8370 73.3134 5 7 -1 -1-81.8456 34.4786 6 7 -1 0 48.7850 33.0356 6 7 -1 1 581.135 50.7026 6 7 -1 2 1951.97 74.3871 6 7 -1 3 390.328 53.2499 6 7 -1 4 160.203 52.9471 6 7 -1 5 284.213 48.5508 6 -7 0 3 1159.46 89.2591 5 -7 0 2 255.885 81.3647 5 7 0 -1 352.592 29.6444 6 7 0 0 31.7862 37.3635 6 7 0 1-44.6099 33.2986 6 7 0 2-49.1512 38.0424 6 7 0 3-10.6920 45.3510 6 7 0 4-104.771 45.6929 6 7 0 5 396.742 51.3937 6 7 0 6 780.822 57.8763 6 -7 -1 3-111.956 61.1133 5 -7 -1 2 1011.34 89.5516 5 7 1 -1 345.067 40.3073 6 -7 -1 1 183.480 73.8537 5 7 1 0 131.719 35.4580 6 7 1 1 525.330 47.3177 6 7 1 2 557.143 49.3201 6 7 1 3 296.844 50.9905 6 7 1 4 93.1790 40.0334 6 7 1 5 155.254 44.2170 6 7 1 6 335.825 58.7649 6 7 1 7 260.345 47.8847 6 -7 -2 2 399.010 79.2290 5 -7 -2 1-72.8496 74.0418 5 7 2 0 38.7153 54.5866 6 7 2 2-32.6927 46.2327 6 7 2 3 148.404 46.0257 6 7 2 4 435.063 48.0965 6 7 2 5-67.9960 46.9955 6 7 2 6 264.740 49.7426 6 7 2 7 733.914 59.7376 6 7 2 8 409.370 46.8775 6 -7 -3 2 34.3733 61.0586 5 -7 -3 1 140.758 59.2781 5 7 3 0 771.330 62.6505 6 7 3 2 183.736 48.0040 6 7 3 3-7.19769 52.4921 6 7 3 4 126.879 49.6608 6 7 3 5 32.1203 57.1468 6 7 3 6-35.4442 56.3378 6 7 3 7 194.082 61.2892 6 7 3 8 63.2736 53.6453 6 -7 -4 1 1231.38 86.2269 5 7 4 0 349.387 55.3243 6 7 4 1 537.210 62.9573 6 7 4 2 1775.94 79.5054 6 7 4 3 1158.28 69.1287 6 7 4 4 218.561 55.6510 6 7 4 5 44.0189 59.4742 6 7 4 7-112.418 53.8072 6 7 4 8 6.52237 61.0987 6 -7 -5 0 96.0240 56.0540 5 7 5 1 654.016 65.6173 6 7 5 2 1007.90 72.9815 6 7 5 3 247.172 58.3996 6 7 5 4 159.439 60.4371 6 7 5 5 32.8676 58.6667 6 7 5 6 97.1099 49.7161 6 7 5 7 85.8507 50.5641 6 -7 -6 0 441.643 83.9235 5 7 6 1 58.8888 59.4312 6 7 6 2 205.451 50.0282 6 7 6 3 610.488 67.8441 6 7 6 4 285.684 56.3920 6 7 6 5 199.708 57.8825 6 7 6 6 383.788 62.6271 6 7 7 2 584.012 69.9798 6 ; _shelx_hkl_checksum 50055 _shelx_res_file ; TITL SPVT2 IN P-1 shelx.res created by SHELXL-2018/3 at 12:15:34 on 24-Jul-2026 CELL 0.71073 6.1050 10.7020 11.8910 63.290 81.600 84.340 ZERR 2.00 0.0004 0.0003 0.0003 0.004 0.003 0.004 LATT 1 SFAC C H N O S UNIT 26 36 4 2 2 MERG 2 OMIT -1 -2 1 OMIT 1 1 0 OMIT -4 0 10 SHEL 12 0.8 DELU 0.001 0.001 C5 C6 DFIX 0.86 0.02 N1 H1N N2 H2N HTAB N1 O1 HTAB N1 O1 EQIV $1 -x+1, -y+1, -z+1 HTAB N2 S1_$1 FMAP 2 PLAN 30 SIZE 0.160 0.480 0.500 ACTA BOND $H CONF LIST 4 L.S. 14 WGHT 0.056100 0.653600 FVAR 7.67414 C1 1 0.653453 0.004130 0.757148 11.00000 0.06564 0.03767 = 0.04732 -0.01290 0.01105 0.01031 C2 1 0.472929 -0.070842 0.778854 11.00000 0.06569 0.04699 = 0.05556 -0.02168 0.00144 0.00942 C3 1 0.409572 -0.170185 0.907377 11.00000 0.08401 0.04918 = 0.05748 -0.01658 0.00963 0.01413 AFIX 43 H3 2 0.285478 -0.223253 0.927043 11.00000 -1.20000 AFIX 0 C4 1 0.531039 -0.186154 0.999499 11.00000 0.09397 0.06217 = 0.05532 -0.01823 0.00659 0.01553 AFIX 43 H4 2 0.486587 -0.250364 1.082242 11.00000 -1.20000 AFIX 0 C5 1 0.714967 -0.112986 0.977166 11.00000 0.10840 0.07443 = 0.04847 -0.01741 -0.01775 0.02149 AFIX 43 H5 2 0.795826 -0.128953 1.043172 11.00000 -1.20000 AFIX 0 C6 1 0.781143 -0.014121 0.854859 11.00000 0.09350 0.06116 = 0.04818 -0.01861 -0.01493 0.02750 AFIX 43 H6 2 0.904989 0.038526 0.837313 11.00000 -1.20000 AFIX 0 C7 1 0.645514 0.236682 0.577806 11.00000 0.04456 0.03526 = 0.03399 -0.01061 -0.00003 0.00045 C8 1 0.941564 0.300141 0.394352 11.00000 0.03684 0.04310 = 0.03851 -0.01606 -0.00101 -0.00044 C9 1 1.028449 0.425401 0.273717 11.00000 0.04295 0.03959 = 0.04135 -0.01391 0.00649 -0.00109 C10 1 0.844125 0.491159 0.186765 11.00000 0.07227 0.06413 = 0.03980 -0.01385 -0.00424 0.00380 AFIX 33 H10A 2 0.722387 0.522879 0.229562 11.00000 -1.50000 H10B 2 0.900447 0.569074 0.110502 11.00000 -1.50000 H10C 2 0.794361 0.422614 0.165898 11.00000 -1.50000 AFIX 0 C11 1 1.106888 0.531513 0.311030 11.00000 0.05921 0.06144 = 0.07604 -0.03171 0.00852 -0.01759 AFIX 33 H11A 2 0.984175 0.562679 0.353691 11.00000 -1.50000 H11B 2 1.219945 0.488307 0.366534 11.00000 -1.50000 H11C 2 1.165792 0.610173 0.236291 11.00000 -1.50000 AFIX 0 C12 1 1.221365 0.375124 0.205993 11.00000 0.06887 0.06068 = 0.06601 -0.01802 0.02959 0.00264 AFIX 33 H12A 2 1.277779 0.453031 0.129752 11.00000 -1.50000 H12B 2 1.336465 0.334007 0.260380 11.00000 -1.50000 H12C 2 1.171636 0.306594 0.185095 11.00000 -1.50000 AFIX 0 C13 1 0.352591 -0.055042 0.678390 11.00000 0.08176 0.06477 = 0.07355 -0.02396 -0.00393 -0.00514 AFIX 33 H13A 2 0.230783 -0.116751 0.712468 11.00000 -1.50000 H13B 2 0.297175 0.039974 0.636992 11.00000 -1.50000 H13C 2 0.449045 -0.077743 0.618279 11.00000 -1.50000 AFIX 0 N1 3 0.728652 0.106180 0.630183 11.00000 0.05269 0.04039 = 0.04071 -0.00877 0.00920 0.00719 N2 3 0.754974 0.327325 0.462090 11.00000 0.04417 0.03545 = 0.03938 -0.00881 0.00583 0.00327 O1 4 1.029248 0.183509 0.429590 11.00000 0.05371 0.04378 = 0.05467 -0.01229 0.00795 0.00944 S1 5 0.422039 0.295577 0.640544 11.00000 0.05729 0.03948 = 0.04821 -0.01245 0.01439 0.00483 H1N 2 0.841209 0.083968 0.592333 11.00000 -1.20000 H2N 2 0.702709 0.411258 0.434276 11.00000 -1.20000 HKLF 4 REM SPVT2 IN P-1 REM wR2 = 0.1639, GooF = S = 1.155, Restrained GooF = 1.156 for all data REM R1 = 0.0641 for 2287 Fo > 4sig(Fo) and 0.0781 for all 2756 data REM 160 parameters refined using 3 restraints END WGHT 0.0561 0.6536 REM Highest difference peak 0.713, deepest hole -0.239, 1-sigma level 0.056 Q1 1 0.2848 -0.1569 0.8205 11.00000 0.05 0.71 Q2 1 0.6329 -0.0460 0.8409 11.00000 0.05 0.63 Q3 1 0.5503 0.0057 0.7084 11.00000 0.05 0.34 Q4 1 0.5580 -0.1266 0.9304 11.00000 0.05 0.32 Q5 1 0.8089 -0.0432 0.8569 11.00000 0.05 0.24 Q6 1 0.7869 -0.0228 0.8963 11.00000 0.05 0.21 Q7 1 1.0193 0.5814 0.3632 11.00000 0.05 0.19 Q8 1 0.9682 0.3670 0.3245 11.00000 0.05 0.19 Q9 1 0.4125 0.0275 0.5806 11.00000 0.05 0.18 Q10 1 1.3376 0.4579 0.1593 11.00000 0.05 0.18 Q11 1 1.3326 0.3630 0.2665 11.00000 0.05 0.18 Q12 1 1.3655 0.3159 0.3161 11.00000 0.05 0.16 Q13 1 0.3985 -0.1486 0.6303 11.00000 0.05 0.16 Q14 1 0.6916 0.0377 0.7407 11.00000 0.05 0.16 Q15 1 0.8397 0.1700 0.8153 11.00000 0.05 0.15 Q16 1 0.3500 -0.1998 0.9642 11.00000 0.05 0.15 Q17 1 0.3946 0.3422 0.5493 11.00000 0.05 0.15 Q18 1 1.1184 0.3844 0.2580 11.00000 0.05 0.15 Q19 1 0.5629 0.2999 0.6613 11.00000 0.05 0.15 Q20 1 0.6957 0.2747 0.5136 11.00000 0.05 0.14 Q21 1 0.5358 0.2816 0.5823 11.00000 0.05 0.14 Q22 1 0.6290 -0.0001 1.0842 11.00000 0.05 0.14 Q23 1 1.1013 0.4840 0.4427 11.00000 0.05 0.14 Q24 1 1.3033 0.2875 0.2457 11.00000 0.05 0.14 Q25 1 1.3378 0.2980 0.4619 11.00000 0.05 0.13 Q26 1 0.5664 -0.2018 0.6339 11.00000 0.05 0.13 Q27 1 0.2169 0.3097 0.6086 11.00000 0.05 0.13 Q28 1 0.5409 -0.1815 0.5615 11.00000 0.05 0.13 Q29 1 0.9508 0.4583 0.2402 11.00000 0.05 0.13 Q30 1 1.2255 0.3149 0.4384 11.00000 0.05 0.13 ; _shelx_res_checksum 33612 loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, -y, -z' loop_ _atom_site_type_symbol _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group C C1 0.6535(6) 0.0041(3) 0.7571(3) 0.0553(8) Uani d 1 . . C C2 0.4729(6) -0.0708(3) 0.7789(3) 0.0582(8) Uani d 1 . . C C3 0.4096(7) -0.1702(4) 0.9074(3) 0.0694(10) Uani d 1 . . H H3 0.285478 -0.223253 0.927043 0.083 Uiso calc 1 . . C C4 0.5310(8) -0.1862(4) 0.9995(4) 0.0765(11) Uani d 1 . . H H4 0.486587 -0.250364 1.082242 0.092 Uiso calc 1 . . C C5 0.7150(8) -0.1130(4) 0.9772(3) 0.0817(12) Uani d 1 . . H H5 0.795826 -0.128953 1.043172 0.098 Uiso calc 1 . . C C6 0.7811(7) -0.0141(4) 0.8549(3) 0.0712(10) Uani d 1 . . H H6 0.904989 0.038526 0.837313 0.085 Uiso calc 1 . . C C7 0.6455(4) 0.2367(3) 0.5778(2) 0.0404(6) Uani d 1 . . C C8 0.9416(4) 0.3001(3) 0.3944(2) 0.0407(6) Uani d 1 . . C C9 1.0284(5) 0.4254(3) 0.2737(3) 0.0441(6) Uani d 1 . . C C10 0.8441(6) 0.4912(4) 0.1868(3) 0.0629(9) Uani d 1 . . H H10A 0.722387 0.522879 0.229562 0.094 Uiso calc 1 . . H H10B 0.900447 0.569074 0.110502 0.094 Uiso calc 1 . . H H10C 0.794361 0.422614 0.165898 0.094 Uiso calc 1 . . C C11 1.1069(6) 0.5315(4) 0.3110(4) 0.0657(9) Uani d 1 . . H H11A 0.984175 0.562679 0.353691 0.099 Uiso calc 1 . . H H11B 1.219945 0.488307 0.366534 0.099 Uiso calc 1 . . H H11C 1.165792 0.610173 0.236291 0.099 Uiso calc 1 . . C C12 1.2214(6) 0.3751(4) 0.2060(4) 0.0735(11) Uani d 1 . . H H12A 1.277779 0.453031 0.129752 0.110 Uiso calc 1 . . H H12B 1.336465 0.334007 0.260380 0.110 Uiso calc 1 . . H H12C 1.171636 0.306594 0.185095 0.110 Uiso calc 1 . . C C13 0.3526(7) -0.0550(4) 0.6784(4) 0.0762(10) Uani d 1 . . H H13A 0.230783 -0.116751 0.712468 0.114 Uiso calc 1 . . H H13B 0.297175 0.039974 0.636992 0.114 Uiso calc 1 . . H H13C 0.449045 -0.077743 0.618279 0.114 Uiso calc 1 . . N N1 0.7287(4) 0.1062(2) 0.6302(2) 0.0503(6) Uani d 1 . . N N2 0.7550(4) 0.3273(2) 0.4621(2) 0.0441(6) Uani d 1 . . O O1 1.0292(3) 0.1835(2) 0.4296(2) 0.0567(6) Uani d 1 . . S S1 0.42204(13) 0.29558(7) 0.64054(7) 0.0537(3) Uani d 1 . . H H1N 0.841(4) 0.084(4) 0.592(3) 0.064 Uiso d 1 . . H H2N 0.703(6) 0.411(2) 0.434(3) 0.064 Uiso d 1 . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 C1 0.066(2) 0.0377(14) 0.0473(16) 0.0103(13) 0.0110(14) -0.0129(12) C2 0.066(2) 0.0470(16) 0.0556(18) 0.0094(15) 0.0014(15) -0.0217(14) C3 0.084(3) 0.0492(18) 0.057(2) 0.0141(17) 0.0096(18) -0.0166(16) C4 0.094(3) 0.062(2) 0.055(2) 0.016(2) 0.007(2) -0.0182(17) C5 0.108(3) 0.074(2) 0.0485(17) 0.021(2) -0.0178(19) -0.0174(15) C6 0.093(3) 0.061(2) 0.0482(16) 0.0275(18) -0.0149(17) -0.0186(13) C7 0.0446(14) 0.0353(13) 0.0340(13) 0.0004(11) 0.0000(11) -0.0106(10) C8 0.0368(13) 0.0431(14) 0.0385(14) -0.0004(11) -0.0010(11) -0.0161(11) C9 0.0429(14) 0.0396(14) 0.0414(14) -0.0011(11) 0.0065(11) -0.0139(11) C10 0.072(2) 0.064(2) 0.0398(16) 0.0038(17) -0.0042(15) -0.0138(15) C11 0.059(2) 0.061(2) 0.076(2) -0.0176(16) 0.0085(17) -0.0317(18) C12 0.069(2) 0.061(2) 0.066(2) 0.0026(17) 0.0296(17) -0.0180(17) C13 0.082(3) 0.065(2) 0.074(2) -0.0051(19) -0.004(2) -0.0240(19) N1 0.0527(14) 0.0404(12) 0.0407(13) 0.0072(11) 0.0092(11) -0.0088(10) N2 0.0442(12) 0.0354(11) 0.0394(12) 0.0033(9) 0.0058(10) -0.0088(10) O1 0.0537(12) 0.0438(11) 0.0547(12) 0.0094(9) 0.0079(10) -0.0123(9) S1 0.0573(5) 0.0395(4) 0.0482(4) 0.0048(3) 0.0144(3) -0.0124(3) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0033 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0061 0.0033 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0106 0.0060 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' S S 0.1246 0.1234 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag C2 C1 C6 . . 122.8(3) ? C2 C1 N1 . . 120.5(3) ? C6 C1 N1 . . 116.7(3) ? C1 C2 C13 . . 121.8(3) ? C1 C2 C3 . . 117.1(3) ? C13 C2 C3 . . 121.1(4) ? C4 C3 C2 . . 119.7(4) ? C4 C3 H3 . . 120.2 ? C2 C3 H3 . . 120.2 ? C3 C4 C5 . . 123.2(4) ? C3 C4 H4 . . 118.4 ? C5 C4 H4 . . 118.4 ? C4 C5 C6 . . 119.4(4) ? C4 C5 H5 . . 120.3 ? C6 C5 H5 . . 120.3 ? C5 C6 C1 . . 117.9(4) ? C5 C6 H6 . . 121.0 ? C1 C6 H6 . . 121.0 ? N1 C7 N2 . . 116.4(2) ? N1 C7 S1 . . 124.4(2) ? N2 C7 S1 . . 119.26(19) ? O1 C8 N2 . . 121.7(2) ? O1 C8 C9 . . 122.8(2) ? N2 C8 C9 . . 115.5(2) ? C12 C9 C8 . . 108.6(2) ? C12 C9 C11 . . 110.0(3) ? C8 C9 C11 . . 108.3(2) ? C12 C9 C10 . . 109.5(3) ? C8 C9 C10 . . 109.9(2) ? C11 C9 C10 . . 110.5(3) ? C9 C10 H10A . . 109.5 ? C9 C10 H10B . . 109.5 ? H10A C10 H10B . . 109.5 ? C9 C10 H10C . . 109.5 ? H10A C10 H10C . . 109.5 ? H10B C10 H10C . . 109.5 ? C9 C11 H11A . . 109.5 ? C9 C11 H11B . . 109.5 ? H11A C11 H11B . . 109.5 ? C9 C11 H11C . . 109.5 ? H11A C11 H11C . . 109.5 ? H11B C11 H11C . . 109.5 ? C9 C12 H12A . . 109.5 ? C9 C12 H12B . . 109.5 ? H12A C12 H12B . . 109.5 ? C9 C12 H12C . . 109.5 ? H12A C12 H12C . . 109.5 ? H12B C12 H12C . . 109.5 ? C2 C13 H13A . . 109.5 ? C2 C13 H13B . . 109.5 ? H13A C13 H13B . . 109.5 ? C2 C13 H13C . . 109.5 ? H13A C13 H13C . . 109.5 ? H13B C13 H13C . . 109.5 ? C7 N1 C1 . . 123.3(2) ? C7 N1 H1N . . 119(2) ? C1 N1 H1N . . 117(2) ? C8 N2 C7 . . 128.5(2) ? C8 N2 H2N . . 118(2) ? C7 N2 H2N . . 114(2) ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag C1 C2 . 1.353(5) ? C1 C6 . 1.424(5) ? C1 N1 . 1.448(4) ? C2 C13 . 1.430(5) ? C2 C3 . 1.436(5) ? C3 C4 . 1.350(6) ? C3 H3 . 0.9300 ? C4 C5 . 1.358(6) ? C4 H4 . 0.9300 ? C5 C6 . 1.388(5) ? C5 H5 . 0.9300 ? C6 H6 . 0.9300 ? C7 N1 . 1.329(3) ? C7 N2 . 1.393(3) ? C7 S1 . 1.665(3) ? C8 O1 . 1.218(3) ? C8 N2 . 1.381(3) ? C8 C9 . 1.525(4) ? C9 C12 . 1.521(4) ? C9 C11 . 1.529(4) ? C9 C10 . 1.536(4) ? C10 H10A . 0.9600 ? C10 H10B . 0.9600 ? C10 H10C . 0.9600 ? C11 H11A . 0.9600 ? C11 H11B . 0.9600 ? C11 H11C . 0.9600 ? C12 H12A . 0.9600 ? C12 H12B . 0.9600 ? C12 H12C . 0.9600 ? C13 H13A . 0.9600 ? C13 H13B . 0.9600 ? C13 H13C . 0.9600 ? N1 H1N . 0.840(18) ? N2 H2N . 0.852(18) ? loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_site_symmetry_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA _geom_hbond_publ_flag N1 H1N O1 . 0.840(18) 1.98(3) 2.644(3) 135(3) yes C11 H11A S1 2_666 0.96 2.79 3.663(4) 152.00 yes C12 H12C Cg1 2_756 0.96 2.92 3.640(5) 133 yes loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion _geom_torsion_publ_flag C6 C1 C2 C13 . . . . -177.3(3) ? N1 C1 C2 C13 . . . . 1.3(5) ? C6 C1 C2 C3 . . . . 1.2(4) ? N1 C1 C2 C3 . . . . 179.8(3) ? C1 C2 C3 C4 . . . . -0.8(5) ? C13 C2 C3 C4 . . . . 177.7(3) ? C2 C3 C4 C5 . . . . -0.6(6) ? C3 C4 C5 C6 . . . . 1.6(6) ? C4 C5 C6 C1 . . . . -1.1(5) ? C2 C1 C6 C5 . . . . -0.3(5) ? N1 C1 C6 C5 . . . . -178.9(3) ? O1 C8 C9 C12 . . . . 4.4(4) ? N2 C8 C9 C12 . . . . -175.6(3) ? O1 C8 C9 C11 . . . . -115.0(3) ? N2 C8 C9 C11 . . . . 65.0(3) ? O1 C8 C9 C10 . . . . 124.2(3) ? N2 C8 C9 C10 . . . . -55.8(3) ? N2 C7 N1 C1 . . . . 171.6(3) ? S1 C7 N1 C1 . . . . -9.1(5) ? C2 C1 N1 C7 . . . . 84.0(4) ? C6 C1 N1 C7 . . . . -97.4(4) ? O1 C8 N2 C7 . . . . 3.5(5) ? C9 C8 N2 C7 . . . . -176.5(3) ? N1 C7 N2 C8 . . . . -0.8(4) ? S1 C7 N2 C8 . . . . 179.9(2) ?