#------------------------------------------------------------------------------ #$Date: 2012-02-03 17:16:24 +0000 (Fri, 03 Feb 2012) $ #$Revision: 32112 $ #$URL: svn://www.crystallography.net/cod/cif/2/21/43/2214360.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2214360 loop_ _publ_author_name 'Kun-Hua Lin' 'Fei-Fei Zhang' 'Zhe-Yin Yu' _publ_section_title ; Bis[4-(dimethylamino)pyridine-\kN]bis(salicylato-\kO)zinc(II) ; _journal_coeditor_code OM2121 _journal_issue 7 _journal_name_full 'Acta Crystallographica Section E' _journal_page_first m1930 _journal_page_last m1930 _journal_volume 63 _journal_year 2007 _chemical_formula_iupac '[Zn (C7 H5 O3)2 (C7 H10 N2)2]' _chemical_formula_moiety 'C28 H30 N4 O6 Zn' _chemical_formula_sum 'C28 H30 N4 O6 Zn' _chemical_formula_weight 583.93 _chemical_name_systematic ; Bis[4-(dimethylamino)pyridine-\kN]bis(salicylato-\kO)zinc(II) ; _space_group_IT_number 15 _symmetry_cell_setting monoclinic _symmetry_space_group_name_Hall '-C 2yc' _symmetry_space_group_name_H-M 'C 1 2/c 1' _atom_sites_solution_hydrogens geom _atom_sites_solution_primary direct _atom_sites_solution_secondary difmap _audit_creation_method SHELXL97 _cell_angle_alpha 90.00 _cell_angle_beta 93.583(8) _cell_angle_gamma 90.00 _cell_formula_units_Z 4 _cell_length_a 19.961(2) _cell_length_b 7.5009(9) _cell_length_c 18.488(2) _cell_measurement_reflns_used 2692 _cell_measurement_temperature 293(2) _cell_measurement_theta_max 23.72 _cell_measurement_theta_min 2.21 _cell_volume 2762.7(5) _computing_cell_refinement 'SAINT (Bruker, 2000)' _computing_data_collection 'APEX2 (Bruker, 2000)' _computing_data_reduction SAINT _computing_molecular_graphics 'SHELXTL (Sheldrick, 2000)' _computing_publication_material SHELXTL _computing_structure_refinement 'SHELXL97 (Sheldrick, 1997)' _computing_structure_solution 'SHELXS97 (Sheldrick, 1997)' _diffrn_ambient_temperature 293(2) _diffrn_measured_fraction_theta_full 0.997 _diffrn_measured_fraction_theta_max 0.997 _diffrn_measurement_device_type 'Bruker SMART APEXII' _diffrn_measurement_method '\f and \w' _diffrn_radiation_monochromator graphite _diffrn_radiation_source 'fine-focus sealed tube' _diffrn_radiation_type MoK\a _diffrn_radiation_wavelength 0.71073 _diffrn_reflns_av_R_equivalents 0.0200 _diffrn_reflns_av_sigmaI/netI 0.0227 _diffrn_reflns_limit_h_max 20 _diffrn_reflns_limit_h_min -23 _diffrn_reflns_limit_k_max 8 _diffrn_reflns_limit_k_min -8 _diffrn_reflns_limit_l_max 21 _diffrn_reflns_limit_l_min -21 _diffrn_reflns_number 6850 _diffrn_reflns_theta_full 25.00 _diffrn_reflns_theta_max 25.00 _diffrn_reflns_theta_min 2.21 _diffrn_standards_number 0 _exptl_absorpt_coefficient_mu 0.937 _exptl_absorpt_correction_T_max 0.8347 _exptl_absorpt_correction_T_min 0.7663 _exptl_absorpt_correction_type none _exptl_crystal_colour colourless _exptl_crystal_density_diffrn 1.404 _exptl_crystal_density_method 'not measured' _exptl_crystal_description block _exptl_crystal_F_000 1216 _exptl_crystal_size_max 0.30 _exptl_crystal_size_mid 0.20 _exptl_crystal_size_min 0.20 _refine_diff_density_max 0.583 _refine_diff_density_min -0.290 _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.036 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 177 _refine_ls_number_reflns 2419 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.036 _refine_ls_R_factor_all 0.0513 _refine_ls_R_factor_gt 0.0419 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'calc w = 1/[\s^2^(Fo^2^)+(0.0463P)^2^+3.8555P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1012 _refine_ls_wR_factor_ref 0.1068 _reflns_number_gt 2032 _reflns_number_total 2419 _reflns_threshold_expression I>2\s(I) _[local]_cod_data_source_file om2121.cif _[local]_cod_data_source_block I _[local]_cod_cif_authors_sg_H-M 'C 2/c' _cod_database_code 2214360 loop_ _symmetry_equiv_pos_as_xyz 'x, y, z' '-x, y, -z+1/2' 'x+1/2, y+1/2, z' '-x+1/2, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y, z-1/2' '-x+1/2, -y+1/2, -z' 'x+1/2, -y+1/2, z-1/2' loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0033 0.0016 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0061 0.0033 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0106 0.0060 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Zn Zn 0.2839 1.4301 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _atom_site_type_symbol _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_refinement_flags _atom_site_occupancy Zn Zn1 0.0000 0.58617(6) 0.2500 0.05591(19) Uani d S 1 C C1 0.15627(14) 0.2514(4) 0.31399(16) 0.0536(7) Uani d . 1 C C2 0.19655(18) 0.2440(5) 0.37794(17) 0.0682(9) Uani d . 1 C C3 0.24291(17) 0.1075(5) 0.38911(19) 0.0709(9) Uani d . 1 H H3 0.2699 0.1028 0.4319 0.085 Uiso calc R 1 C C4 0.24888(16) -0.0184(5) 0.3378(2) 0.0734(9) Uani d . 1 H H4 0.2803 -0.1091 0.3456 0.088 Uiso calc R 1 C C5 0.20952(17) -0.0147(5) 0.2746(2) 0.0783(10) Uani d . 1 H H5 0.2138 -0.1026 0.2397 0.094 Uiso calc R 1 C C6 0.16372(15) 0.1199(4) 0.26335(18) 0.0642(8) Uani d . 1 H H6 0.1370 0.1223 0.2203 0.077 Uiso calc R 1 C C7 0.10649(19) 0.3990(5) 0.3030(3) 0.0789(10) Uani d . 1 C C8 -0.01148(16) 0.9075(4) 0.15743(17) 0.0649(8) Uani d . 1 H H8 -0.0528 0.9157 0.1778 0.078 Uiso calc R 1 C C9 0.00609(16) 1.0410(4) 0.11356(16) 0.0625(8) Uani d . 1 H H9 -0.0228 1.1372 0.1051 0.075 Uiso calc R 1 C C10 0.06755(15) 1.0362(4) 0.08056(14) 0.0532(7) Uani d . 1 C C11 0.10614(15) 0.8820(4) 0.09559(16) 0.0566(7) Uani d . 1 H H11 0.1466 0.8665 0.0740 0.068 Uiso calc R 1 C C12 0.08467(14) 0.7553(4) 0.14149(15) 0.0543(7) Uani d . 1 H H12 0.1122 0.6570 0.1510 0.065 Uiso calc R 1 C C13 0.0484(2) 1.3291(5) 0.0261(2) 0.0835(11) Uani d . 1 H H13A 0.0519 1.4051 0.0670 0.100 Uiso d R 1 H H13B 0.0638 1.3916 -0.0158 0.100 Uiso d R 1 H H13C 0.0013 1.2988 0.0151 0.100 Uiso d R 1 C C14 0.1501(2) 1.1575(6) 0.0028(2) 0.0967(13) Uani d . 1 H H14A 0.1476 1.0874 -0.0415 0.116 Uiso d R 1 H H14B 0.1679 1.2744 -0.0092 0.116 Uiso d R 1 H H14C 0.1871 1.1006 0.0343 0.116 Uiso d R 1 N N1 0.02661(12) 0.7628(3) 0.17384(12) 0.0555(6) Uani d . 1 N N2 0.08845(14) 1.1690(4) 0.03907(14) 0.0683(7) Uani d . 1 O O1 0.07388(13) 0.4073(3) 0.24406(18) 0.0930(8) Uani d . 1 O O2 0.09803(19) 0.5057(5) 0.3525(2) 0.1405(14) Uani d . 1 O O3 0.1925(2) 0.3681(5) 0.43048(16) 0.1324(13) Uani d . 1 H H3A 0.1616 0.4356 0.4193 0.159 Uiso d R 1 loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Zn1 0.0570(3) 0.0546(3) 0.0565(3) 0.000 0.0065(2) 0.000 C1 0.0468(15) 0.0503(17) 0.0651(18) -0.0040(13) 0.0138(13) 0.0031(14) C2 0.079(2) 0.069(2) 0.0574(19) -0.0070(8) 0.0153(16) -0.0098(16) C3 0.065(2) 0.083(2) 0.063(2) -0.0058(18) -0.0032(15) 0.0084(18) C4 0.0552(19) 0.071(2) 0.094(3) 0.0100(17) 0.0049(18) 0.003(2) C5 0.070(2) 0.075(2) 0.089(3) 0.0123(19) 0.0035(19) -0.027(2) C6 0.0551(18) 0.075(2) 0.0624(18) -0.0047(16) 0.0005(14) -0.0051(16) C7 0.064(2) 0.065(2) 0.109(3) 0.0015(18) 0.017(2) 0.016(2) C8 0.0542(17) 0.075(2) 0.0675(19) 0.0148(16) 0.0160(14) 0.0046(17) C9 0.0636(19) 0.0623(19) 0.0620(19) 0.0193(15) 0.0068(15) 0.0026(15) C10 0.0603(17) 0.0541(17) 0.0449(15) 0.0057(13) 0.0027(13) -0.0044(13) C11 0.0536(16) 0.0557(18) 0.0617(17) 0.0072(13) 0.0126(13) 0.0016(14) C12 0.0521(16) 0.0525(17) 0.0583(17) 0.0098(13) 0.0047(13) -0.0018(13) C13 0.108(3) 0.061(2) 0.083(2) 0.018(2) 0.011(2) 0.0116(19) C14 0.097(3) 0.086(3) 0.111(3) 0.005(2) 0.039(2) 0.029(2) N1 0.0513(13) 0.0581(15) 0.0575(14) 0.0068(11) 0.0074(11) 0.0015(11) N2 0.0818(18) 0.0587(16) 0.0663(16) 0.0107(14) 0.0193(14) 0.0111(13) O1 0.0681(15) 0.0830(18) 0.127(2) 0.0055(13) -0.0008(16) 0.0269(16) O2 0.159(3) 0.104(2) 0.081(3) 0.043(3) 0.006(3) -0.030(2) O3 0.187(4) 0.121(3) 0.087(2) 0.036(2) -0.008(2) -0.0484(19) loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance Zn1 O1 2 2.002(3) Zn1 O1 . 2.002(3) Zn1 N1 . 2.028(2) Zn1 N1 2 2.028(2) C1 C6 . 1.375(4) C1 C2 . 1.389(4) C1 C7 . 1.493(5) C2 O3 . 1.351(4) C2 C3 . 1.387(5) C3 C4 . 1.349(5) C3 H3 . 0.9300 C4 C5 . 1.367(5) C4 H4 . 0.9300 C5 C6 . 1.369(5) C5 H5 . 0.9300 C6 H6 . 0.9300 C7 O1 . 1.235(5) C7 O2 . 1.236(5) C8 N1 . 1.349(4) C8 C9 . 1.349(4) C8 H8 . 0.9300 C9 C10 . 1.404(4) C9 H9 . 0.9300 C10 N2 . 1.340(4) C10 C11 . 1.408(4) C11 C12 . 1.361(4) C11 H11 . 0.9300 C12 N1 . 1.338(3) C12 H12 . 0.9300 C13 N2 . 1.454(4) C13 H13A . 0.9460 C13 H13B . 0.9719 C13 H13C . 0.9775 C14 N2 . 1.440(4) C14 H14A . 0.9714 C14 H14B . 0.9769 C14 H14C . 1.0073 O3 H3A . 0.8156 loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle O1 Zn1 O1 2 . 95.82(15) O1 Zn1 N1 2 . 134.57(12) O1 Zn1 N1 . . 100.02(10) O1 Zn1 N1 2 2 100.02(10) O1 Zn1 N1 . 2 134.57(12) N1 Zn1 N1 . 2 98.43(14) C6 C1 C2 . . 118.0(3) C6 C1 C7 . . 122.6(3) C2 C1 C7 . . 119.4(3) O3 C2 C3 . . 118.1(3) O3 C2 C1 . . 121.8(3) C3 C2 C1 . . 120.1(3) C4 C3 C2 . . 120.0(3) C4 C3 H3 . . 120.0 C2 C3 H3 . . 120.0 C3 C4 C5 . . 121.1(3) C3 C4 H4 . . 119.5 C5 C4 H4 . . 119.5 C4 C5 C6 . . 119.1(3) C4 C5 H5 . . 120.4 C6 C5 H5 . . 120.4 C5 C6 C1 . . 121.7(3) C5 C6 H6 . . 119.1 C1 C6 H6 . . 119.1 O1 C7 O2 . . 122.1(4) O1 C7 C1 . . 117.9(4) O2 C7 C1 . . 120.0(4) N1 C8 C9 . . 124.6(3) N1 C8 H8 . . 117.7 C9 C8 H8 . . 117.7 C8 C9 C10 . . 120.6(3) C8 C9 H9 . . 119.7 C10 C9 H9 . . 119.7 N2 C10 C9 . . 122.8(3) N2 C10 C11 . . 122.5(3) C9 C10 C11 . . 114.7(3) C12 C11 C10 . . 120.5(3) C12 C11 H11 . . 119.8 C10 C11 H11 . . 119.8 N1 C12 C11 . . 124.4(3) N1 C12 H12 . . 117.8 C11 C12 H12 . . 117.8 N2 C13 H13A . . 110.7 N2 C13 H13B . . 109.4 H13A C13 H13B . . 109.7 N2 C13 H13C . . 110.7 H13A C13 H13C . . 109.2 H13B C13 H13C . . 107.1 N2 C14 H14A . . 115.1 N2 C14 H14B . . 112.7 H14A C14 H14B . . 107.2 N2 C14 H14C . . 111.9 H14A C14 H14C . . 104.8 H14B C14 H14C . . 104.4 C12 N1 C8 . . 115.2(3) C12 N1 Zn1 . . 123.7(2) C8 N1 Zn1 . . 120.88(19) C10 N2 C14 . . 121.9(3) C10 N2 C13 . . 121.4(3) C14 N2 C13 . . 116.7(3) C7 O1 Zn1 . . 109.6(3) C2 O3 H3A . . 108.9 loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA _geom_hbond_publ_flag O3 H3A O2 0.82 1.79 2.522(5) 148 y