#------------------------------------------------------------------------------ #$Date: 2022-11-05 02:51:29 +0000 (Sat, 05 Nov 2022) $ #$Revision: 278947 $ #$URL: svn://www.crystallography.net/cod/cif/2/24/42/2244202.cif $ #------------------------------------------------------------------------------ # # This file is available in the Crystallography Open Database (COD), # http://www.crystallography.net/. The original data for this entry # were provided by IUCr Journals, http://journals.iucr.org/. # # The file may be used within the scientific community so long as # proper attribution is given to the journal article from which the # data were obtained. # data_2244202 loop_ _publ_author_name 'Kamolov, Sanjar' 'Babaev, Bakhrom' 'Ibragimov, Aziz' 'Yakubov, Yuldash' 'Abdullaev, Akhrorjon' 'Ibragimov, Bakhtiyar' 'Ashurov, Jamshid' _publ_section_title ; Synthesis, structure and Hirshfeld surface analysis of diaquadinitratobis(4-nitroaniline)copper(II) ; _journal_coeditor_code YZ2022 _journal_issue 12 _journal_name_full 'Acta Crystallographica Section E' _journal_page_first ; ; _journal_paper_doi 10.1107/S2056989022010404 _journal_volume 78 _journal_year 2022 _chemical_formula_iupac '[Cu (N O3)2 (C6 H6 N2 O2)2 (H2 O)2]' _chemical_formula_moiety 'C12 H16 Cu N6 O12' _chemical_formula_sum 'C12 H16 Cu N6 O12' _chemical_formula_weight 499.86 _chemical_name_systematic ; Diaquadinitratobis(4-nitroaniline)copper(II) ; _space_group_crystal_system monoclinic _space_group_IT_number 14 _space_group_name_Hall '-P 2ybc' _space_group_name_H-M_alt 'P 1 21/c 1' _atom_sites_solution_hydrogens mixed _atom_sites_solution_primary dual _atom_sites_solution_secondary difmap _audit_creation_method ; Olex2 1.5 (compiled 2022.04.07 svn.rca3783a0 for OlexSys, GUI svn.r6498) ; _cell_angle_alpha 90 _cell_angle_beta 92.286(3) _cell_angle_gamma 90 _cell_formula_units_Z 2 _cell_length_a 5.4741(2) _cell_length_b 22.5679(6) _cell_length_c 7.6478(2) _cell_measurement_reflns_used 2724 _cell_measurement_temperature 293(2) _cell_measurement_theta_max 70.1780 _cell_measurement_theta_min 3.9040 _cell_volume 944.05(5) _computing_cell_refinement ; CrysAlisPro (Rigaku OD, 2020) ; _computing_data_collection ; CrysAlisPro (Rigaku OD, 2020) ; _computing_data_reduction ; CrysAlisPro (Rigaku OD, 2020) ; _computing_molecular_graphics ; Mercury (Macrae et al., 2020) ; _computing_publication_material ; publCIF (Westrip, 2010) ; _computing_structure_refinement ; SHELXL2019/2 (Sheldrick, 2015b) ; _computing_structure_solution ; SHELXT2018/2 (Sheldrick, 2015a) ; _diffrn_ambient_temperature 293(2) _diffrn_detector 'Hybrid Pixel Array Detector' _diffrn_detector_area_resol_mean 10.0000 _diffrn_measured_fraction_theta_full 1.000 _diffrn_measured_fraction_theta_max 0.992 _diffrn_measurement_device 'four-circle diffractometer' _diffrn_measurement_device_type 'XtaLAB Synergy, Single source at home/near, HyPix3000' _diffrn_measurement_method '\w scans' _diffrn_radiation_monochromator mirror _diffrn_radiation_probe x-ray _diffrn_radiation_type 'Cu K\a' _diffrn_radiation_wavelength 1.54184 _diffrn_reflns_av_R_equivalents 0.0621 _diffrn_reflns_av_unetI/netI 0.0481 _diffrn_reflns_limit_h_max 6 _diffrn_reflns_limit_h_min -6 _diffrn_reflns_limit_k_max 19 _diffrn_reflns_limit_k_min -27 _diffrn_reflns_limit_l_max 9 _diffrn_reflns_limit_l_min -9 _diffrn_reflns_number 8364 _diffrn_reflns_theta_full 67.684 _diffrn_reflns_theta_max 71.518 _diffrn_reflns_theta_min 3.918 _diffrn_source 'micro-focus sealed X-ray tube' _exptl_absorpt_coefficient_mu 2.382 _exptl_absorpt_correction_T_max 1.00000 _exptl_absorpt_correction_T_min 0.82883 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details ; (CrysAlisPro; Rigaku OD, 2020) ; _exptl_crystal_colour 'metallic greenish green' _exptl_crystal_density_diffrn 1.758 _exptl_crystal_description needle _exptl_crystal_F_000 510 _exptl_crystal_size_max 0.18 _exptl_crystal_size_mid 0.15 _exptl_crystal_size_min 0.14 _refine_diff_density_max 0.523 _refine_diff_density_min -0.872 _refine_ls_extinction_coef 0.0033(5) _refine_ls_extinction_expression Fc^*^=kFc[1+0.001xFc^2^\l^3^/sin(2\q)]^-1/4^ _refine_ls_extinction_method ; SHELXL-2019/2 (Sheldrick 2015a) ; _refine_ls_goodness_of_fit_ref 1.042 _refine_ls_hydrogen_treatment mixed _refine_ls_matrix_type full _refine_ls_number_parameters 159 _refine_ls_number_reflns 1832 _refine_ls_number_restraints 0 _refine_ls_restrained_S_all 1.042 _refine_ls_R_factor_all 0.0579 _refine_ls_R_factor_gt 0.0449 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0573P)^2^+0.7131P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1140 _refine_ls_wR_factor_ref 0.1232 _reflns_number_gt 1457 _reflns_number_total 1832 _reflns_threshold_expression 'I > 2\s(I)' _cod_data_source_file yz2022sup1.cif _cod_data_source_block I _cod_database_code 2244202 _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _shelx_estimated_absorpt_t_min 0.674 _shelx_estimated_absorpt_t_max 0.731 _shelx_hkl_file ; 0 0 -1 -0.22 0.72 0 0 1 -0.22 0.84 0 0 2 2699.79 132.54 0 0 2 2771.48 134.21 0 0 -2 2854.88 132.75 0 0 3 -1.05 2.59 0 0 4 6.16 4.67 0 0 -5 4.76 5.50 0 0 5 -2.13 4.92 0 0 5 -1.88 4.03 0 0 5 7.59 6.63 0 0 -6 437.35 39.80 0 0 6 548.27 44.35 0 0 6 480.51 37.97 0 0 -7 -3.93 6.86 0 0 -7 -3.24 7.49 0 0 -8 2.77 6.86 0 0 -8 13.60 7.87 0 0 9 2.70 3.73 0 0 -9 2.05 3.59 0 0 -9 3.33 4.11 0 1 1 1220.88 61.73 0 -1 1 1318.20 63.25 0 1 -1 1310.18 61.80 0 1 1 1334.99 63.22 0 -1 1 1273.27 62.88 0 -1 1 1359.98 62.11 0 -1 1 1297.45 63.16 0 -1 1 1328.91 63.03 0 -1 -1 1359.59 63.08 0 -1 -2 247.94 15.22 0 1 -2 222.16 13.90 0 -1 2 226.33 15.11 0 -1 2 255.55 15.35 0 1 2 225.21 13.93 0 -1 2 273.28 16.50 0 1 2 257.37 16.17 0 -1 3 357.13 24.45 0 1 3 400.52 25.20 0 -1 3 386.74 23.24 0 -1 -3 329.09 22.54 0 1 4 7.69 5.06 0 -1 4 13.88 5.58 0 1 5 1259.98 76.64 0 -1 5 1239.78 72.24 0 1 5 1291.94 74.26 0 -1 5 1356.01 77.58 0 1 -5 1123.59 73.43 0 -1 -5 1164.33 74.24 0 1 6 19.09 9.65 0 1 6 21.41 7.80 0 -1 -6 9.01 6.97 0 -1 6 9.80 6.08 0 1 -6 8.85 7.31 0 -1 6 3.16 9.16 0 1 -7 25.76 10.28 0 -1 -7 54.46 15.30 0 1 -7 35.53 13.02 0 -1 -7 39.17 11.88 0 1 -8 -6.85 7.92 0 -1 -8 -3.35 7.17 0 -1 8 4.56 5.27 0 -1 -8 2.79 7.32 0 1 -8 2.75 5.88 0 -1 -9 41.83 8.48 0 1 9 27.31 6.42 0 1 -9 20.81 7.80 0 -1 9 23.69 5.87 0 1 -9 14.63 5.44 0 -1 -9 39.75 9.26 0 -2 0 2421.38 111.52 0 -2 0 2448.61 112.24 0 -2 0 2419.17 112.01 0 -2 0 2325.47 111.11 0 -2 0 2338.67 111.52 0 -2 0 2267.61 111.68 0 -2 0 2415.28 111.68 0 -2 0 2444.66 111.40 0 -2 1 8.43 1.85 0 -2 1 11.27 2.17 0 -2 1 11.45 2.27 0 2 1 12.81 2.09 0 -2 -1 12.06 2.75 0 -2 -1 9.15 1.97 0 -2 1 13.23 2.40 0 -2 1 13.46 2.00 0 -2 1 13.64 2.34 0 -2 2 3194.72 153.27 0 -2 2 3120.17 153.43 0 -2 -2 3244.14 153.68 0 2 2 3233.94 154.00 0 -2 2 3201.58 153.98 0 -2 3 920.65 48.92 0 2 3 862.67 48.42 0 -2 -3 822.51 47.08 0 -2 3 857.18 47.08 0 2 4 23.14 6.17 0 -2 4 40.27 7.89 0 -2 4 26.68 6.48 0 -2 5 91.52 13.38 0 -2 -5 118.79 14.52 0 -2 5 83.03 13.00 0 2 5 97.49 16.06 0 -2 5 75.79 14.04 0 -2 -5 97.59 16.58 0 2 -5 87.20 14.41 0 -2 -5 65.34 13.16 0 2 -6 185.32 23.60 0 2 6 211.29 26.00 0 2 6 217.78 22.82 0 -2 -6 184.34 24.30 0 -2 6 176.94 21.46 0 2 -7 50.88 12.87 0 -2 -7 45.76 12.59 0 -2 -7 19.20 9.67 0 2 7 55.50 14.34 0 2 -7 51.42 14.78 0 -2 -8 -3.27 5.72 0 -2 8 6.71 5.18 0 -2 -8 19.54 8.45 0 2 -8 5.38 6.65 0 2 -8 3.42 7.32 0 2 9 -1.36 2.91 0 2 -9 -4.15 5.44 0 -2 9 3.78 3.30 0 -2 -9 1.89 4.94 0 -2 -9 1.67 3.85 0 2 -9 -1.57 3.62 0 -3 0 0.13 0.58 0 -3 0 -0.41 0.71 0 -3 0 -0.18 0.67 0 -3 0 0.23 0.66 0 -3 0 0.99 1.25 0 -3 0 0.29 1.09 0 -3 0 -0.25 0.72 0 3 1 262.19 14.91 0 -3 -1 261.05 15.86 0 -3 1 276.32 15.07 0 -3 1 284.24 15.51 0 -3 -1 268.18 16.05 0 -3 1 278.65 15.83 0 -3 -1 273.53 16.51 0 -3 1 274.18 15.93 0 -3 1 250.17 15.51 0 -3 2 1225.05 60.47 0 3 2 1204.33 60.06 0 -3 -2 1206.66 60.36 0 -3 2 1113.02 60.14 0 -3 2 1211.35 59.97 0 -3 2 1187.58 60.04 0 -3 -2 1053.94 61.56 0 -3 3 886.79 47.34 0 -3 3 796.20 46.53 0 -3 3 834.77 46.11 0 3 3 885.37 47.32 0 -3 -3 870.82 46.61 0 -3 -4 214.07 21.94 0 3 4 247.99 20.63 0 -3 4 229.23 20.13 0 -3 4 190.69 18.47 0 -3 -5 774.33 56.74 0 -3 5 891.62 53.83 0 -3 -5 810.45 55.70 0 -3 5 787.27 52.75 0 -3 -5 882.36 53.90 0 3 5 805.62 56.15 0 3 -5 696.95 52.85 0 -3 6 7.52 6.57 0 -3 -6 2.48 4.86 0 3 6 9.66 7.96 0 -3 -6 3.06 7.56 0 -3 6 7.58 5.42 0 -3 -6 10.45 7.46 0 3 -6 2.92 5.11 0 -3 -7 158.14 24.39 0 -3 -7 160.67 23.19 0 -3 -7 163.42 20.87 0 3 -7 150.29 22.08 0 3 -7 138.17 23.52 0 3 7 173.25 23.81 0 3 -8 39.21 10.89 0 3 -8 27.08 10.00 0 -3 -8 63.54 13.58 0 -3 -8 37.85 11.20 0 -3 8 52.20 11.09 0 -3 -9 21.24 5.91 0 3 -9 10.36 4.69 0 3 9 5.35 4.40 0 3 -9 8.15 5.36 0 -4 0 3408.44 156.25 0 -4 0 3246.34 154.89 0 -4 0 3305.16 156.62 0 -4 0 3305.36 155.41 0 -4 0 3373.28 155.21 0 -4 0 3243.79 154.29 0 -4 0 3298.95 155.23 0 -4 0 3234.61 155.62 0 -4 1 698.14 34.53 0 -4 -1 718.03 35.70 0 -4 1 658.12 33.07 0 -4 1 668.83 34.34 0 -4 1 684.62 34.49 0 -4 1 681.67 34.72 0 -4 -1 644.95 34.61 0 -4 -1 608.88 34.60 0 4 1 596.85 32.81 0 4 2 458.34 28.44 0 -4 -2 503.96 31.24 0 -4 2 517.91 29.73 0 -4 2 538.02 29.29 0 -4 2 536.85 30.03 0 -4 -2 529.96 30.05 0 -4 3 2622.69 124.12 0 -4 -3 2519.95 123.77 0 -4 3 2589.96 123.91 0 4 3 2322.46 123.04 0 -4 3 2425.27 123.90 0 -4 -3 2323.57 125.98 0 -4 -4 368.47 30.94 0 -4 -4 400.01 28.43 0 -4 4 418.20 29.45 0 4 4 379.05 28.57 0 -4 4 396.78 28.13 0 -4 4 369.14 28.35 0 -4 -5 145.11 19.12 0 4 5 176.62 21.31 0 -4 -5 151.00 18.00 0 -4 -5 147.22 20.50 0 -4 5 172.71 19.07 0 4 -5 103.81 16.45 0 -4 5 144.00 17.32 0 4 -6 252.66 28.04 0 -4 -6 273.83 27.59 0 -4 -6 283.28 30.00 0 4 6 298.82 31.74 0 -4 6 284.46 27.71 0 -4 6 257.81 27.11 0 4 -7 3.92 7.67 0 -4 -7 5.39 6.66 0 -4 7 2.60 5.56 0 4 -7 3.07 6.01 0 4 7 3.45 7.40 0 -4 -7 3.27 6.38 0 -4 8 4.19 5.81 0 -4 -8 13.62 7.91 0 4 -8 23.25 9.20 0 4 -8 12.60 6.63 0 4 -9 -1.97 4.21 0 4 9 -1.30 3.21 0 -4 -9 -1.58 3.38 0 -5 0 -0.50 2.19 0 -5 0 -1.12 2.51 0 -5 0 -0.34 1.48 0 -5 0 1.09 1.13 0 -5 0 -0.39 1.59 0 -5 0 -0.43 1.58 0 -5 0 1.09 1.42 0 -5 1 2196.66 103.85 0 -5 -1 2105.12 103.92 0 -5 1 2184.69 101.36 0 -5 1 2216.99 101.44 0 -5 1 2163.16 103.71 0 -5 1 2153.87 103.79 0 -5 1 2172.02 103.46 0 -5 1 2176.00 103.37 0 5 1 1759.90 100.86 0 -5 -1 2141.47 103.73 0 -5 1 2237.74 102.11 0 -5 -1 2372.33 105.08 0 -5 2 412.90 24.18 0 -5 -2 364.08 23.59 0 -5 -2 364.00 24.79 0 -5 2 373.06 23.56 0 5 2 318.54 21.73 0 -5 2 405.06 22.85 0 -5 2 397.24 23.88 0 5 3 2.15 2.83 0 -5 3 4.69 3.25 0 -5 3 1.22 3.20 0 -5 -3 7.66 5.19 0 -5 3 4.34 3.80 0 -5 -3 4.82 3.50 0 -5 4 62.90 9.74 0 5 4 53.41 8.96 0 -5 -4 51.25 9.02 0 -5 4 59.94 10.00 0 -5 4 57.57 9.49 0 -5 -4 39.91 10.06 0 -5 4 71.35 10.33 0 5 5 596.10 47.01 0 -5 -5 610.59 44.57 0 -5 5 692.30 45.38 0 -5 5 656.78 45.68 0 -5 -5 653.93 48.49 0 -5 -5 685.02 48.23 0 -5 6 2.59 4.54 0 -5 -6 3.10 8.99 0 -5 6 5.27 4.61 0 5 6 -3.27 7.56 0 -5 -6 -2.64 6.10 0 -5 -7 243.70 26.44 0 5 -7 217.15 26.64 0 5 -7 217.35 29.57 0 -5 -7 270.00 29.49 0 5 7 270.89 30.28 0 -5 -8 -2.65 6.96 0 5 -8 -3.23 6.91 0 5 9 9.89 4.20 0 5 -9 3.72 4.61 0 -5 -9 7.49 4.36 0 -6 0 748.10 38.52 0 -6 0 715.56 38.99 0 -6 0 769.90 38.43 0 -6 0 742.31 38.75 0 -6 0 758.00 39.91 0 -6 0 785.33 40.68 0 -6 1 3201.80 154.19 0 -6 -1 3045.85 154.64 0 -6 -1 3301.52 154.40 0 -6 1 3201.38 151.81 0 -6 -1 3254.19 154.42 0 -6 1 3219.18 151.98 0 -6 1 3364.94 154.64 0 -6 -1 3066.98 154.31 0 -6 1 3225.11 154.63 0 -6 1 3110.62 153.46 0 -6 2 161.68 12.03 0 -6 -2 138.54 12.76 0 -6 2 140.35 12.61 0 -6 2 152.88 12.71 0 -6 -2 144.04 13.64 0 -6 2 166.29 13.19 0 -6 2 134.72 11.56 0 -6 3 580.69 36.64 0 -6 3 717.12 39.69 0 -6 -3 603.28 40.02 0 -6 3 605.02 38.22 0 -6 -3 596.43 38.26 0 -6 4 526.28 35.33 0 -6 -4 478.93 34.43 0 -6 4 472.55 33.52 0 -6 4 506.42 35.27 0 -6 -4 467.46 36.63 0 -6 5 31.85 8.19 0 -6 -5 31.77 8.97 0 -6 5 30.04 9.13 0 -6 -5 31.30 9.49 0 6 5 19.16 8.39 0 -6 5 24.92 8.50 0 -6 6 523.07 40.57 0 -6 6 515.14 41.17 0 -6 -6 471.55 40.20 0 6 6 417.88 40.64 0 -6 -6 564.01 44.77 0 6 7 -3.39 6.62 0 -6 -7 3.21 8.43 0 6 -7 -3.82 6.67 0 6 -8 102.43 18.38 0 -6 -8 97.66 15.60 0 -6 -9 5.58 3.66 0 6 9 5.79 3.66 0 6 -9 1.72 4.25 0 -7 0 -0.53 1.59 0 -7 0 -0.49 1.73 0 -7 0 3.29 3.13 0 -7 0 1.13 1.97 0 -7 0 0.62 2.32 0 -7 0 1.46 2.71 0 -7 1 346.74 22.42 0 -7 1 347.44 21.19 0 -7 -1 338.71 21.78 0 -7 1 351.91 21.80 0 -7 -1 348.69 22.57 0 -7 -1 333.06 22.06 0 -7 1 358.48 22.30 0 -7 -2 109.73 11.38 0 -7 2 116.50 10.39 0 -7 -2 138.68 13.18 0 -7 2 127.63 11.33 0 -7 2 113.83 11.78 0 -7 2 115.65 11.43 0 -7 2 129.08 11.85 0 -7 3 706.12 44.10 0 -7 3 744.73 43.04 0 -7 -3 705.55 44.51 0 -7 -3 753.73 46.79 0 -7 3 763.09 44.87 0 -7 4 3.26 3.77 0 -7 -4 6.61 5.45 0 -7 -4 3.73 4.31 0 -7 4 5.41 4.46 0 -7 4 3.67 3.94 0 -7 -5 205.52 21.80 0 7 5 122.96 19.75 0 -7 5 149.62 18.78 0 -7 5 178.38 20.59 0 -7 5 205.13 22.61 0 -7 -5 178.26 22.12 0 -7 -6 -6.29 6.74 0 -7 6 10.08 6.61 0 -7 6 5.30 5.18 0 -7 -6 5.56 7.29 0 7 6 19.84 10.42 0 7 -7 227.10 30.37 0 7 7 243.26 28.92 0 -7 -8 2.45 6.07 0 7 -8 2.95 5.15 0 7 9 40.28 6.95 0 -7 9 60.85 8.43 0 7 -9 36.83 7.88 0 -7 -9 49.29 7.87 0 -8 0 1395.00 70.98 0 -8 0 1373.55 69.89 0 -8 0 1374.31 71.82 0 -8 0 1362.76 69.27 0 -8 1 288.57 20.06 0 -8 -1 279.26 20.18 0 -8 -1 302.55 20.41 0 -8 1 307.05 19.25 0 -8 1 302.45 20.61 0 -8 -1 251.36 19.14 0 -8 1 298.21 19.72 0 -8 2 956.04 51.29 0 -8 -2 789.56 50.68 0 -8 2 927.38 50.96 0 -8 2 919.78 51.52 0 -8 -2 1017.62 53.87 0 -8 -3 322.22 24.87 0 -8 3 301.02 23.59 0 -8 3 281.11 23.38 0 -8 -3 314.18 25.62 0 -8 4 1164.88 69.24 0 -8 4 1237.50 69.79 0 -8 4 1228.46 68.05 0 -8 -4 1205.33 71.69 0 -8 -4 1043.54 68.16 0 -8 -5 22.12 8.64 0 -8 5 22.70 8.30 0 8 5 11.43 7.95 0 -8 -5 29.85 9.82 0 -8 5 17.72 7.04 0 -8 -6 289.70 29.15 0 -8 -6 267.54 29.92 0 -8 6 268.76 28.67 0 8 6 209.06 27.71 0 -8 6 308.38 29.02 0 -8 7 -2.48 4.84 0 -8 -7 -3.08 6.03 0 8 7 3.25 6.36 0 -8 7 5.45 5.83 0 8 -7 3.60 7.70 0 8 -8 57.73 12.93 0 -8 -8 92.60 14.84 0 -9 0 -2.24 3.24 0 -9 0 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9.01 5 -4 -1 6.41 7.41 -5 -4 1 -2.57 5.49 5 4 -1 -2.86 5.60 5 -4 -1 -2.86 6.61 5 4 0 202.70 27.94 5 -4 0 321.05 31.45 -5 -4 0 292.30 30.86 -5 -4 0 373.45 30.76 5 4 0 234.88 27.05 5 -4 0 289.04 29.36 5 4 1 13.64 8.50 -5 4 -1 21.48 11.34 -5 -4 -1 31.82 11.18 -5 4 -1 21.47 9.35 5 4 1 25.65 9.71 5 -4 1 31.37 9.71 5 4 2 9.86 8.16 -5 4 -2 32.64 12.70 -5 4 -2 8.41 7.78 -5 4 -2 16.94 9.39 5 -4 2 22.25 9.65 -5 -4 -3 -2.54 5.43 -5 4 -3 6.46 8.93 5 -4 3 -3.02 5.90 5 4 3 -2.99 5.85 -5 -4 -4 60.88 11.92 -5 4 -4 70.54 13.95 -5 4 -4 43.66 11.09 5 -4 4 57.55 12.76 5 4 4 41.94 11.27 -5 -4 -5 5.12 4.48 -5 4 -5 8.26 5.41 5 -4 5 11.75 6.64 5 -5 -6 20.87 5.72 5 5 -6 13.95 5.54 -5 -5 6 14.02 4.64 -5 5 6 12.95 4.42 5 -5 -5 133.98 16.83 5 -5 -5 130.41 17.21 5 5 -5 113.56 17.35 -5 5 5 121.48 14.98 5 -5 -4 2.85 6.11 -5 -5 4 2.10 4.49 -5 5 4 -2.10 4.85 5 -5 -3 95.44 17.67 -5 -5 3 112.95 16.03 -5 5 3 78.67 13.30 5 -5 -2 29.54 11.18 -5 -5 2 25.39 8.96 5 -5 -1 12.97 8.51 -5 -5 1 23.13 8.41 5 5 -1 2.80 6.01 5 -5 -1 2.79 5.99 5 5 0 215.91 27.95 5 -5 0 302.50 30.77 -5 -5 0 273.27 29.43 -5 -5 0 236.54 25.66 5 5 0 269.18 27.84 5 -5 0 271.70 27.92 5 5 1 64.16 14.31 -5 5 -1 82.80 17.61 -5 5 -1 66.43 15.14 5 5 1 105.75 16.72 5 -5 1 80.76 14.45 5 5 2 61.25 14.71 -5 5 -2 64.99 16.70 -5 5 -2 64.61 15.76 5 -5 2 82.98 15.75 -5 -5 -3 96.82 17.45 -5 5 -3 154.12 21.97 5 -5 3 122.53 19.41 5 5 3 86.88 16.60 -5 -5 -4 45.59 10.74 -5 5 -4 36.00 10.45 -5 5 -4 31.21 9.74 5 -5 4 40.31 10.50 5 5 4 58.42 11.71 -5 -5 -5 30.98 7.32 -5 5 -5 32.87 7.68 5 -5 5 52.45 9.97 5 -6 -6 26.55 6.56 5 6 -6 33.58 7.58 -5 -6 6 46.30 7.68 -5 6 6 40.61 6.79 5 -6 -5 22.82 7.61 5 -6 -5 29.72 8.62 -5 -6 5 35.26 9.17 5 6 -5 35.53 10.03 -5 6 5 31.29 7.47 5 -6 -4 110.56 17.46 -5 -6 4 123.67 15.70 -5 6 4 92.13 14.12 5 -6 -3 9.40 8.67 -5 -6 3 9.35 6.79 5 -6 -2 13.10 9.09 -5 -6 2 25.06 8.80 5 -6 -2 15.96 7.40 5 -6 -1 179.59 24.68 -5 -6 1 179.27 21.78 5 -6 -1 159.87 21.36 5 6 0 136.06 21.95 5 -6 0 142.36 21.84 -5 -6 0 136.67 20.85 5 -6 0 130.51 19.25 5 6 1 99.83 17.95 5 -6 1 83.62 15.52 -5 6 -1 50.46 15.08 -5 6 -1 47.35 12.77 5 6 2 112.98 19.23 -5 6 -2 96.56 20.12 -5 -6 -2 105.00 18.46 -5 -6 -3 16.68 7.33 -5 6 -3 18.99 9.21 5 -6 3 39.14 10.96 5 6 3 8.32 6.46 -5 -6 -4 31.08 8.60 -5 6 -4 26.91 9.79 5 -6 4 28.80 9.24 -5 6 -4 27.87 8.49 -5 -6 -5 -3.08 3.56 -5 6 -5 1.46 3.38 5 -6 5 5.28 4.35 5 -7 -6 3.86 3.37 -5 -7 6 1.23 3.03 -5 7 6 -1.99 2.31 5 -7 -5 112.32 14.90 5 -7 -5 124.33 15.60 -5 -7 5 118.61 15.14 -5 7 5 95.38 12.58 5 -7 -4 13.24 7.68 -5 -7 4 2.46 3.74 -5 7 4 5.67 5.23 5 -7 -3 94.90 17.84 -5 -7 3 117.00 16.50 5 -7 -2 -3.25 7.50 -5 -7 2 2.45 4.79 -5 -7 2 2.52 5.40 5 -7 -1 19.61 11.12 -5 -7 1 25.35 9.46 5 7 0 60.40 14.56 -5 7 0 24.32 11.60 -5 -7 0 44.07 12.53 5 7 1 78.10 15.89 5 -7 1 75.59 15.04 -5 7 -1 61.02 15.37 -5 -7 -1 65.12 14.57 -5 7 -1 60.58 13.70 5 7 2 6.06 7.01 -5 7 -2 3.52 8.71 -5 -7 -2 12.49 7.72 -5 7 -3 48.19 14.78 -5 -7 -3 56.63 12.02 -5 7 -3 46.41 12.62 -5 -7 -4 5.85 5.12 -5 7 -4 10.35 6.79 5 -7 4 8.98 5.89 -5 7 -4 2.04 5.36 -5 -7 -5 48.29 9.21 -5 -7 -5 59.92 9.30 -5 7 -5 40.14 7.59 5 -7 5 64.63 10.17 5 -8 -5 1.85 4.29 -5 -8 5 3.72 3.64 -5 8 5 -1.41 2.76 5 -8 -4 127.78 18.42 -5 -8 4 153.05 18.97 5 -8 -3 8.89 7.77 -5 -8 3 -2.55 4.98 -5 -8 3 -2.14 4.18 5 -8 -2 31.90 12.19 -5 -8 2 19.02 7.83 -5 -8 2 15.21 7.73 5 -8 -1 3.25 7.51 -5 -8 1 -4.98 4.87 5 8 0 3.28 7.06 5 -8 0 19.15 9.68 -5 8 0 24.29 11.36 -5 -8 0 21.74 9.81 5 8 1 12.62 7.82 5 -8 1 6.07 7.98 -5 8 -1 10.66 9.83 -5 -8 -1 31.99 10.84 -5 8 -1 8.38 6.00 -5 -8 -2 374.31 34.34 5 8 2 303.49 31.36 -5 8 -2 296.27 33.89 -5 8 -3 18.56 10.12 -5 -8 -3 5.19 5.56 -5 -8 -3 5.03 5.82 -5 8 -3 3.00 6.93 -5 -8 -4 6.39 4.94 -5 -8 -4 14.45 5.92 -5 8 -4 2.45 4.81 -5 8 -4 7.67 5.57 5 -8 5 7.21 3.66 -5 -8 -5 5.99 3.49 5 -9 -5 12.01 5.24 -5 -9 5 17.29 5.89 5 -9 -4 23.32 8.93 -5 -9 4 17.81 6.80 5 -9 -3 175.70 22.12 -5 -9 3 145.54 18.92 5 -9 -2 15.53 9.46 -5 -9 2 20.51 8.03 -5 -9 2 30.28 9.67 5 -9 -1 121.66 20.00 -5 -9 1 121.94 17.97 5 9 0 38.23 12.75 5 -9 0 63.34 14.64 -5 9 0 55.02 14.67 -5 -9 0 91.33 15.98 5 9 1 3.02 5.29 5 -9 1 15.11 9.15 -5 9 -1 3.49 9.15 -5 -9 -1 3.12 8.19 -5 9 -2 3.34 8.26 -5 -9 -2 -2.95 6.31 -5 -9 -2 2.61 5.58 -5 9 -3 29.46 11.04 -5 -9 -3 27.24 8.25 -5 -9 -3 46.29 10.55 -5 9 -3 34.40 10.45 -5 -9 -3 37.40 9.04 -5 -9 -4 -2.02 4.32 -5 9 -4 2.29 5.31 -5 9 -4 -1.78 4.11 -5 -9 -5 66.79 9.66 -5 -9 -5 51.18 7.99 5 -10 -5 1.56 3.61 5 -10 -5 -1.47 3.41 -5 -10 5 4.74 3.65 -5 -10 5 2.92 4.24 5 -10 -4 31.91 8.37 -5 -10 4 52.00 10.17 -5 -10 4 61.37 11.14 5 -10 -3 10.69 7.77 -5 -10 3 11.58 7.03 5 -10 -2 50.84 13.15 -5 -10 2 79.51 14.05 5 -10 -1 -3.12 7.22 -5 -10 1 2.53 5.41 5 10 0 30.53 10.82 5 -10 0 74.67 15.49 -5 10 0 47.31 14.28 -5 -10 0 29.62 9.14 -5 -10 0 37.14 10.31 5 10 1 -2.86 7.50 5 -10 1 -2.97 6.88 -5 10 -1 -3.40 8.40 -5 -10 -1 3.03 5.29 -5 10 -2 154.10 24.35 -5 -10 -2 195.71 22.66 -5 10 -3 -2.77 7.67 -5 -10 -3 2.34 4.57 -5 -10 -3 -2.33 4.56 -5 10 -3 -2.71 5.80 -5 -10 -3 4.01 5.26 5 -10 4 22.51 6.03 -5 -10 -4 28.26 7.60 -5 10 -4 25.28 7.87 -5 10 -4 11.31 5.37 -5 -10 -5 9.66 4.11 5 -11 -5 18.40 5.35 -5 -11 5 21.15 5.73 -5 -11 5 23.64 6.04 5 -11 -4 18.75 6.97 -5 -11 4 7.65 4.45 -5 -11 4 9.26 5.86 5 -11 -3 228.06 24.24 5 -11 -3 213.29 22.57 -5 -11 3 206.22 22.14 5 -11 -2 70.99 14.79 -5 -11 2 86.03 14.54 -5 -11 2 99.06 15.30 5 -11 -1 135.37 19.81 -5 -11 1 136.48 18.59 5 11 0 25.96 9.59 5 -11 0 42.30 12.23 -5 11 0 36.15 12.96 -5 -11 0 60.00 12.61 -5 -11 0 34.21 9.47 5 -11 1 78.11 14.78 -5 11 -1 65.52 16.42 -5 -11 -1 43.62 11.40 -5 11 -2 12.20 8.45 -5 -11 -2 8.06 5.29 -5 -11 -2 26.95 8.59 -5 11 -3 41.21 11.10 -5 -11 -3 61.00 11.40 -5 -11 -3 63.93 11.69 -5 11 -3 52.89 11.72 -5 -11 -3 59.22 11.00 5 -11 4 4.40 4.44 -5 -11 -4 -3.46 3.70 -5 11 -4 -1.89 3.30 -5 11 -4 -2.87 3.76 -5 -12 5 -1.22 2.39 -5 -12 5 2.27 2.98 5 -12 -4 70.04 11.11 -5 -12 4 69.04 10.80 -5 -12 4 62.91 10.65 5 -12 -3 143.96 18.09 5 -12 -3 116.98 16.20 -5 -12 3 137.95 17.25 5 -12 -2 26.52 8.82 -5 -12 2 48.17 10.07 -5 -12 2 32.44 9.63 5 -12 -1 79.99 15.27 -5 -12 1 71.93 13.08 -5 -12 1 50.51 11.12 5 -12 0 193.85 23.81 -5 -12 0 158.12 20.70 -5 -12 0 149.87 18.92 -5 12 -1 -3.12 7.71 -5 -12 -1 2.76 4.83 5 -12 2 143.97 16.86 -5 -12 -2 186.69 21.36 -5 -12 -2 153.86 18.93 -5 -12 -2 147.82 17.94 -5 12 -3 4.70 6.16 5 -12 3 13.74 5.62 -5 -12 -3 11.99 6.05 -5 -12 -3 2.05 3.11 -5 12 -3 -2.30 5.31 -5 -12 -3 7.16 4.95 5 -12 4 3.92 3.63 -5 12 -4 4.91 4.54 5 -13 -4 18.29 5.89 -5 -13 4 30.35 6.84 -5 -13 4 16.34 5.74 -5 -13 4 24.33 6.59 5 -13 -3 250.72 23.33 -5 -13 3 247.86 22.96 -5 -13 3 251.33 23.42 5 -13 -2 12.14 6.72 5 -13 -2 8.04 5.29 -5 -13 2 6.25 5.17 -5 -13 2 17.48 7.41 5 -13 -1 130.67 18.69 -5 -13 1 118.95 16.49 -5 -13 1 165.19 19.42 5 -13 0 13.64 7.92 -5 13 0 5.99 9.08 -5 -13 0 9.12 5.66 -5 13 -1 46.83 12.87 -5 -13 -1 77.69 13.71 -5 -13 -1 66.22 12.16 -5 13 -2 2.63 6.09 -5 -13 -2 9.34 5.77 -5 -13 -2 2.18 4.27 -5 13 -2 2.52 4.93 -5 -13 -2 2.06 4.76 -5 13 -3 39.80 10.45 5 -13 3 55.39 9.41 -5 -13 -3 67.42 11.22 -5 13 -3 28.58 8.11 -5 -13 -3 77.33 11.01 5 -13 4 24.86 5.77 -5 -13 -4 20.23 5.75 5 -14 -4 160.00 15.36 -5 -14 4 159.32 15.39 -5 -14 4 157.57 15.32 5 -14 -3 -1.70 3.32 -5 -14 3 1.70 4.21 -5 -14 3 -1.75 4.04 5 -14 -2 12.99 6.00 5 -14 -2 18.43 6.66 -5 -14 2 1.95 4.52 -5 -14 2 14.16 7.30 5 -14 -1 -2.44 4.76 5 -14 -1 -2.11 4.12 -5 -14 1 -2.04 4.73 -5 -14 1 -2.15 4.60 -5 14 0 86.56 16.53 -5 -14 0 118.74 15.58 -5 14 -1 -2.70 6.68 -5 -14 -1 -4.16 5.14 -5 14 -2 76.07 14.02 -5 -14 -2 88.27 13.46 -5 14 -2 63.30 12.48 -5 -14 -2 116.44 14.56 5 -14 3 -1.34 3.32 -5 -14 -3 -1.67 4.13 -5 14 -3 3.50 4.05 -5 -14 -3 1.48 3.41 5 -15 -3 75.94 10.63 -5 -15 3 75.91 10.98 -5 -15 3 67.45 10.50 5 -15 -2 3.70 5.36 5 -15 -2 1.65 3.54 -5 -15 2 7.11 5.60 -5 -15 2 -1.83 4.52 5 -15 -1 180.54 18.85 -5 -15 1 147.59 17.14 -5 -15 1 136.14 17.06 5 -15 0 13.07 5.69 -5 15 0 10.22 7.76 -5 -15 0 12.84 5.35 -5 -15 0 18.71 6.97 -5 15 -1 85.43 15.17 -5 -15 -1 132.15 15.48 -5 15 -2 2.09 5.17 -5 15 -2 -1.96 3.84 -5 -15 -2 -3.35 4.39 5 -15 3 13.48 4.07 -5 -15 -3 4.33 3.81 -5 -15 -3 8.97 4.06 5 -16 -3 10.77 4.73 5 -16 -3 11.35 4.43 -5 -16 3 7.82 3.97 -5 -16 3 6.44 4.23 5 -16 -2 173.28 17.53 5 -16 -2 146.71 15.70 -5 -16 2 172.31 17.18 -5 -16 2 171.47 17.08 5 -16 -1 3.49 4.32 -5 -16 1 -1.71 3.66 5 -16 0 62.46 10.29 -5 16 0 45.69 11.11 -5 -16 0 72.95 11.15 -5 16 -1 2.15 5.94 -5 -16 -1 1.62 3.74 -5 16 -2 21.32 7.18 -5 -16 -2 20.22 6.13 5 -17 -2 12.54 4.74 -5 17 2 4.70 4.77 -5 -17 2 13.54 4.90 5 -17 -1 123.27 13.90 -5 -17 1 136.08 14.36 5 -17 0 28.09 7.12 -5 17 0 5.95 6.53 -5 17 -1 36.56 9.33 -5 -17 -1 53.79 8.65 -5 17 -1 19.68 6.63 -5 -17 -1 46.90 7.95 -5 -17 -2 -1.23 2.40 -5 -17 -2 1.19 2.74 5 -18 -1 11.42 4.60 -5 18 1 6.32 5.38 -5 -18 1 17.51 5.38 5 -18 0 30.93 6.40 -5 18 0 37.91 8.30 -5 -18 0 34.10 6.83 -5 18 -1 10.29 5.30 -5 -18 -1 4.65 3.06 6 0 -4 1.48 3.17 -6 0 4 -2.43 3.01 6 0 -4 -1.43 3.54 -6 0 3 -3.09 4.68 6 0 -3 -1.84 3.22 -6 0 2 65.61 10.87 6 0 -2 82.13 13.06 -6 0 1 11.30 6.85 -6 0 1 3.53 4.88 6 0 -1 -2.24 4.80 -6 0 0 308.51 28.08 6 0 0 269.07 25.93 6 0 0 257.62 26.38 6 0 1 2.37 5.07 6 0 2 17.25 6.84 -6 0 -3 -1.63 3.49 6 0 3 -3.51 4.06 6 -1 -4 1.51 3.23 6 1 -4 -1.43 3.30 -6 -1 4 -1.21 3.18 -6 1 4 -2.40 3.32 6 1 -4 1.42 3.04 6 -1 -4 1.42 2.48 6 -1 -3 7.49 5.24 -6 -1 3 21.80 6.43 -6 1 3 22.74 6.12 6 1 -3 14.63 5.36 6 -1 -3 23.73 6.43 -6 -1 2 -1.75 4.33 -6 1 2 -3.36 3.29 6 1 -2 4.19 4.49 6 -1 -2 -2.09 3.66 6 1 -1 98.20 15.47 -6 -1 1 111.08 15.88 -6 1 1 100.34 15.39 -6 -1 1 99.37 13.85 6 1 -1 80.34 13.49 6 -1 -1 133.75 16.63 6 1 0 -9.83 6.45 -6 -1 0 7.07 6.18 -6 1 0 -2.37 5.49 6 1 0 -4.50 5.21 6 -1 0 -2.25 4.82 -6 1 -1 18.03 7.37 6 -1 1 4.62 4.96 6 1 1 2.40 5.95 6 -1 2 2.11 4.88 6 1 2 4.34 5.36 -6 -1 -3 43.79 9.04 -6 1 -3 51.39 8.56 6 -1 3 53.68 9.73 6 1 3 52.56 9.35 6 -2 -4 -1.51 3.96 -6 -2 4 8.32 3.89 -6 2 4 1.16 2.49 6 2 -4 2.76 2.70 6 -2 -4 1.38 2.69 6 -2 -3 -3.79 4.69 -6 -2 3 1.55 4.06 -6 2 3 -1.47 3.39 6 2 -3 1.79 3.13 6 -2 -3 3.57 3.49 -6 -2 2 35.18 7.69 -6 2 2 40.47 8.03 6 2 -2 26.77 7.79 6 -2 -2 30.81 8.17 6 2 -1 38.13 10.52 -6 -2 1 38.95 9.57 -6 2 1 34.23 9.48 -6 -2 1 42.06 9.03 6 2 -1 32.95 9.13 6 -2 -1 17.53 7.57 -6 2 0 254.29 25.04 6 2 0 239.20 23.83 6 -2 0 249.89 24.12 6 2 0 188.78 22.70 -6 2 -1 4.43 5.13 6 -2 1 8.90 5.51 6 2 1 2.41 5.96 6 -2 2 42.92 9.51 6 2 2 36.64 9.28 -6 -2 -3 4.79 3.97 -6 2 -3 15.38 5.20 6 -2 3 18.44 5.69 6 2 3 5.17 5.01 6 -3 -4 8.94 4.52 -6 -3 4 13.73 4.36 -6 3 4 1.11 2.91 6 3 -4 9.21 3.99 6 -3 -4 11.77 4.28 6 -3 -3 5.69 5.25 -6 -3 3 6.09 4.43 -6 3 3 15.38 5.06 6 3 -3 8.65 4.80 6 -3 -3 8.60 4.77 6 3 -2 10.71 7.01 6 -3 -2 10.49 6.36 -6 -3 2 5.24 4.33 -6 3 2 3.97 5.21 6 3 -2 4.00 3.91 6 -3 -2 1.99 4.27 6 3 -1 62.36 12.33 -6 3 1 65.65 12.66 6 3 -1 79.07 12.84 6 -3 -1 87.34 13.34 6 3 0 2.48 6.14 -6 3 0 9.27 6.72 -6 3 -1 56.22 11.55 -6 -3 -1 60.66 12.13 6 3 1 71.58 13.01 -6 -3 -2 10.19 5.93 6 -3 2 7.79 5.67 6 3 2 19.09 7.20 -6 -3 -3 18.67 5.78 -6 3 -3 5.54 3.86 6 -3 3 7.98 4.44 6 3 3 11.67 5.27 6 -4 -4 75.07 10.58 -6 -4 4 66.81 8.41 -6 4 4 50.54 7.40 6 4 -4 48.72 7.97 6 -4 -4 50.77 8.12 6 -4 -3 3.74 5.17 -6 -4 3 2.95 3.42 6 4 -3 9.83 4.53 6 -4 -3 3.25 3.49 6 4 -2 2.15 4.60 6 -4 -2 10.47 6.60 -6 -4 2 8.58 4.98 -6 4 2 7.87 5.16 6 4 -2 1.91 3.35 6 -4 -2 1.90 3.33 6 4 -1 23.86 8.17 -6 4 1 26.72 8.11 6 4 -1 18.46 6.33 6 -4 -1 46.97 9.85 -6 4 0 192.45 21.69 6 4 0 181.32 21.56 6 4 1 4.68 6.46 -6 4 -1 -2.09 5.48 -6 -4 -1 6.59 5.08 -6 -4 -2 7.93 5.22 -6 4 -2 11.37 5.33 6 4 2 12.33 6.24 -6 -4 -3 20.97 5.43 -6 4 -3 12.20 4.62 6 -4 3 10.39 4.53 6 4 3 7.92 4.63 6 -5 -4 12.35 4.52 -6 -5 4 10.86 3.70 6 5 -3 77.24 11.43 6 -5 -3 80.03 12.05 -6 -5 3 78.78 10.47 6 -5 -3 58.68 9.80 6 5 -2 6.38 5.88 6 -5 -2 8.26 6.26 -6 5 2 5.79 6.09 6 5 -2 5.38 3.85 6 -5 -2 5.35 4.41 6 5 -1 28.16 8.71 6 -5 -1 40.32 9.86 -6 5 1 62.95 11.73 6 5 -1 52.30 9.95 6 -5 -1 52.03 9.90 6 5 0 -2.39 5.92 -6 5 0 -2.19 5.42 6 5 1 34.04 9.44 -6 5 -1 40.00 9.70 -6 -5 -1 29.81 8.47 -6 -5 -2 21.03 6.97 -6 5 -2 25.46 6.75 6 5 2 21.60 7.36 -6 -5 -3 18.50 5.47 -6 5 -3 13.72 5.21 -6 5 -3 11.76 4.77 6 5 3 23.57 6.09 6 -6 -4 66.27 9.16 6 6 -3 58.90 10.19 6 -6 -3 68.01 10.96 6 6 -2 49.79 10.61 6 -6 -2 80.49 12.73 -6 6 2 52.40 10.44 6 6 -1 4.56 5.28 6 -6 -1 6.27 4.84 -6 6 1 10.47 6.86 6 6 0 43.91 10.38 -6 6 0 20.99 7.23 6 6 1 4.34 5.69 -6 6 -1 -1.89 4.67 -6 -6 -1 -2.05 3.58 -6 6 -2 1.86 3.99 -6 6 -2 4.62 4.26 6 6 2 7.38 5.59 -6 -6 -3 -1.33 2.33 -6 6 -3 -1.47 3.64 -6 6 -3 -1.24 3.06 6 6 3 2.66 3.08 6 7 -3 27.52 7.59 6 -7 -3 67.39 10.34 6 7 -2 9.98 6.30 6 -7 -2 13.53 6.33 -6 7 2 5.38 4.45 6 7 -1 52.48 11.22 6 -7 -1 69.12 11.75 -6 7 1 37.99 9.21 6 7 0 11.01 6.09 6 -7 0 3.90 4.52 -6 7 0 3.98 5.22 6 7 1 24.49 8.17 -6 7 -1 40.51 9.01 -6 -7 -1 50.58 10.07 -6 7 -1 42.11 10.07 -6 -7 -2 6.88 4.26 -6 7 -2 3.59 4.72 6 7 2 10.16 5.34 -6 -7 -3 25.65 5.60 -6 7 -3 12.55 4.62 -6 7 -3 13.81 4.45 6 8 -3 -1.52 3.53 6 -8 -3 -3.03 3.98 6 -8 -2 170.07 17.83 -6 8 2 137.13 15.89 6 8 -2 130.27 16.28 6 8 -1 -4.13 5.42 6 -8 -1 -5.85 4.82 -6 8 1 -1.88 4.66 6 8 0 2.06 5.41 6 -8 0 -3.77 4.95 -6 8 0 -5.57 4.30 6 8 1 7.52 5.46 -6 8 -1 4.83 4.23 -6 -8 -1 7.31 4.53 -6 8 -1 5.79 4.48 -6 -8 -2 35.18 7.34 -6 8 -2 20.46 6.59 -6 -8 -2 27.33 6.22 6 8 2 16.67 5.41 6 9 -3 16.81 5.41 6 -9 -3 23.17 6.26 6 9 -2 3.50 3.43 6 -9 -2 1.70 3.64 -6 9 2 1.57 3.89 6 9 -1 68.93 11.79 6 -9 -1 102.98 13.73 -6 9 1 68.24 11.39 6 9 0 -1.90 4.06 -6 9 0 -1.71 3.65 -6 -9 -1 69.45 10.84 -6 9 -1 51.19 9.75 6 9 1 40.69 8.59 -6 -9 -2 1.46 2.86 -6 9 -2 1.58 3.66 -6 -9 -2 1.21 2.80 6 10 -2 61.89 10.14 -6 10 2 61.63 10.02 6 10 -1 1.74 3.39 6 -10 -1 1.70 4.46 -6 10 1 1.59 3.94 6 10 0 -1.70 3.32 -6 10 0 6.14 5.36 -6 -10 -1 16.96 5.10 -6 10 -1 15.26 5.97 -6 10 -2 28.69 6.45 -6 -10 -2 36.10 6.45 6 11 -2 4.17 3.23 6 -11 -2 16.24 5.17 -6 11 2 8.90 4.02 6 11 -1 35.05 7.60 -6 11 1 36.89 7.52 6 11 0 10.27 4.45 -6 11 0 9.38 4.98 -6 11 0 3.24 3.48 -6 11 -1 30.65 7.19 -6 -11 -1 48.45 7.81 -6 12 1 -1.22 3.37 -6 12 0 10.10 4.78 -6 -12 0 27.02 5.87 0 0 0 0.00 0.00 TITL exp_257-pnitroanilin+ccu+22 in P2(1)/c REM P2(1)/c (#14 in standard setting) CELL 1.54184 5.474133 22.567859 7.647796 90.0000 92.2858 90.0000 ZERR 4.00 0.000161 0.000552 0.000233 0.0000 0.0028 0.0000 LATT 1 SYMM -x, y+1/2,-z+1/2 SFAC C H N O UNIT 44.00 40.00 4.00 4.00 TREF HKLF 4 END _computing_structure_solution 'SHELXT 2018/2 (Sheldrick, 2018)' _computing_structure_solution 'SHELXT 2018/2 (Sheldrick, 2018)' _computing_structure_solution 'SHELXT 2018/2 (Sheldrick, 2018)' _computing_structure_solution 'SHELXT 2018/2 (Sheldrick, 2018)' _computing_structure_solution 'SHELXT 2018/2 (Sheldrick, 2018)' ; _shelx_hkl_checksum 5687 _shelx_res_file ; TITL exp_257-pnitroanilin+ccu+22.09_a.res in P2(1)/c exp_257-pnitroanilin+ccu+22.09.res created by SHELXL-2019/2 at 09:26:36 on 01-Jul-2022 REM Old TITL exp_257-pnitroanilin+ccu+22.09_a.res in P2(1)/c REM SHELXT solution in P2(1)/c: R1 0.143, Rweak 0.005, Alpha 0.040 REM 0.286 for 63 systematic absences, Orientation as input REM Formula found by SHELXT: C16 Cu N2 O12 CELL 1.54184 5.4741 22.5679 7.6478 90 92.286 90 ZERR 4 0.0002 0.0006 0.0002 0 0.003 0 LATT 1 SYMM -X,0.5+Y,0.5-Z SFAC C H Cu N O UNIT 24 32 2 12 24 L.S. 4 0 0 PLAN 5 SIZE 0.18 0.15 0.14 CONF list 4 MORE -1 BOND $H fmap 2 53 acta REM REM REM WGHT 0.057300 0.713100 EXTI 0.003324 FVAR 0.74288 CU01 3 0.500000 0.500000 0.500000 10.50000 0.03078 0.01542 = 0.03236 -0.00050 0.00460 -0.00180 O1W 5 0.691193 0.570833 0.429966 11.00000 0.04461 0.02038 = 0.04986 0.00127 0.01688 -0.00210 N1 4 0.666924 0.453930 0.306058 11.00000 0.03773 0.02176 = 0.02868 -0.00013 0.00081 -0.00192 O3 5 0.147872 0.526753 0.328317 11.00000 0.03773 0.07967 = 0.03134 0.01107 0.00265 -0.00086 O4 5 0.345787 0.538190 0.093230 11.00000 0.05812 0.06958 = 0.03973 0.01315 0.01675 0.01472 N3 4 0.159588 0.545970 0.172500 11.00000 0.03562 0.03969 = 0.03524 0.00061 -0.00336 0.00285 C1 1 0.611867 0.392647 0.277122 11.00000 0.03400 0.02147 = 0.02942 -0.00355 0.00600 -0.00183 O2 5 0.558141 0.176311 0.242683 11.00000 0.17570 0.02856 = 0.08827 -0.00195 0.03442 0.00146 O5 5 -0.018735 0.571338 0.108582 11.00000 0.05428 0.12443 = 0.07922 0.02002 -0.01559 0.03891 C6 1 0.400471 0.378301 0.179711 11.00000 0.04393 0.03087 = 0.03889 -0.00432 0.00050 -0.00313 AFIX 43 H6 2 0.300983 0.408167 0.132632 11.00000 -1.20000 AFIX 0 N2 4 0.415561 0.214260 0.193398 11.00000 0.12119 0.03826 = 0.06119 -0.01147 0.03558 -0.01666 C2 1 0.761408 0.349178 0.347358 11.00000 0.04341 0.03080 = 0.04579 -0.00305 0.00217 0.00569 AFIX 43 H2 2 0.901766 0.358992 0.413589 11.00000 -1.20000 AFIX 0 C4 1 0.487588 0.277032 0.222856 11.00000 0.07434 0.02741 = 0.04673 -0.01097 0.01930 -0.01502 C5 1 0.338998 0.320167 0.153203 11.00000 0.05618 0.04113 = 0.04913 -0.01332 0.00415 -0.01844 AFIX 43 H5 2 0.197557 0.310181 0.088452 11.00000 -1.20000 AFIX 0 C3 1 0.698409 0.289690 0.317295 11.00000 0.07798 0.02782 = 0.05500 0.00677 0.01812 0.01835 AFIX 43 H3 2 0.798430 0.259361 0.360899 11.00000 -1.20000 AFIX 0 O1 5 0.216734 0.204594 0.118579 11.00000 0.13811 0.05904 = 0.14631 -0.03625 -0.00170 -0.04488 H1A 2 0.627679 0.473993 0.219665 11.00000 0.03203 H1B 2 0.818149 0.460920 0.334323 11.00000 0.05314 H1WA 2 0.812690 0.564883 0.376140 11.00000 0.07492 H1WB 2 0.620867 0.594537 0.378543 11.00000 0.07116 HKLF 4 REM exp_257-pnitroanilin+ccu+22.09_a.res in P2(1)/c REM wR2 = 0.1232, GooF = S = 1.042, Restrained GooF = 1.042 for all data REM R1 = 0.0449 for 1457 Fo > 4sig(Fo) and 0.0579 for all 1832 data REM 159 parameters refined using 0 restraints END WGHT 0.0573 0.7145 REM Highest difference peak 0.523, deepest hole -0.872, 1-sigma level 0.075 Q1 1 0.7281 0.1790 0.3192 11.00000 0.05 0.52 Q2 1 0.5659 0.1968 0.2225 11.00000 0.05 0.33 Q3 1 0.5939 0.2143 0.2418 11.00000 0.05 0.33 Q4 1 0.6444 0.5556 0.2992 11.00000 0.05 0.26 Q5 1 0.3516 0.5398 0.4332 11.00000 0.05 0.26 ; _shelx_res_checksum 45136 loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y-1/2, z-1/2' loop_ _atom_site_type_symbol _atom_site_label _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_calc_flag _atom_site_occupancy _atom_site_disorder_assembly _atom_site_disorder_group Cu Cu1 0.500000 0.500000 0.500000 0.0261(2) Uani d 1 . . O O1W 0.6912(5) 0.57083(11) 0.4300(4) 0.0379(6) Uani d 1 . . N N1 0.6669(6) 0.45393(11) 0.3061(4) 0.0294(6) Uani d 1 . . O O3 0.1479(4) 0.52675(14) 0.3283(3) 0.0495(7) Uani d 1 . . O O4 0.3458(5) 0.53819(13) 0.0932(4) 0.0554(7) Uani d 1 . . N N3 0.1596(5) 0.54597(13) 0.1725(4) 0.0370(6) Uani d 1 . . C C1 0.6119(6) 0.39265(13) 0.2771(4) 0.0282(6) Uani d 1 . . O O2 0.5581(9) 0.17631(14) 0.2427(5) 0.0967(14) Uani d 1 . . O O5 -0.0187(6) 0.57134(19) 0.1086(5) 0.0865(12) Uani d 1 . . C C6 0.4005(6) 0.37830(15) 0.1797(5) 0.0379(8) Uani d 1 . . H H6 0.300983 0.408167 0.132632 0.046 Uiso calc 1 . . N N2 0.4156(10) 0.21426(17) 0.1934(6) 0.0727(13) Uani d 1 . . C C2 0.7614(7) 0.34918(15) 0.3474(5) 0.0400(8) Uani d 1 . . H H2 0.901766 0.358992 0.413589 0.048 Uiso calc 1 . . C C4 0.4876(8) 0.27703(16) 0.2229(5) 0.0490(10) Uani d 1 . . C C5 0.3390(8) 0.32017(17) 0.1532(5) 0.0488(9) Uani d 1 . . H H5 0.197557 0.310181 0.088452 0.059 Uiso calc 1 . . C C3 0.6984(9) 0.28969(16) 0.3173(6) 0.0532(11) Uani d 1 . . H H3 0.798430 0.259361 0.360899 0.064 Uiso calc 1 . . O O1 0.2167(10) 0.20459(17) 0.1186(7) 0.1147(17) Uani d 1 . . H H1A 0.628(7) 0.4740(17) 0.220(5) 0.032(9) Uiso d 1 . . H H1B 0.818(8) 0.4609(19) 0.334(6) 0.053(13) Uiso d 1 . . H H1WA 0.813(10) 0.565(2) 0.376(7) 0.075(17) Uiso d 1 . . H H1WB 0.621(10) 0.595(3) 0.379(7) 0.071(18) Uiso d 1 . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_12 _atom_site_aniso_U_13 _atom_site_aniso_U_23 Cu1 0.0308(4) 0.0154(3) 0.0324(4) -0.0018(2) 0.0046(2) -0.0005(2) O1W 0.0446(15) 0.0204(11) 0.0499(15) -0.0021(10) 0.0169(12) 0.0013(10) N1 0.0377(15) 0.0218(12) 0.0287(14) -0.0019(11) 0.0008(12) -0.0001(11) O3 0.0377(13) 0.0797(19) 0.0313(13) -0.0009(13) 0.0027(10) 0.0111(12) O4 0.0581(16) 0.0696(19) 0.0397(15) 0.0147(14) 0.0168(12) 0.0132(13) N3 0.0356(15) 0.0397(15) 0.0352(15) 0.0028(12) -0.0034(12) 0.0006(12) C1 0.0340(16) 0.0215(14) 0.0294(15) -0.0018(12) 0.0060(12) -0.0035(12) O2 0.176(4) 0.0286(16) 0.088(3) 0.001(2) 0.034(3) -0.0019(17) O5 0.0543(19) 0.124(3) 0.079(2) 0.039(2) -0.0156(17) 0.020(2) C6 0.0439(19) 0.0309(17) 0.0389(18) -0.0031(15) 0.0005(15) -0.0043(14) N2 0.121(4) 0.038(2) 0.061(3) -0.017(2) 0.036(3) -0.0115(18) C2 0.0434(19) 0.0308(17) 0.046(2) 0.0057(15) 0.0022(16) -0.0030(15) C4 0.074(3) 0.0274(18) 0.047(2) -0.0150(18) 0.019(2) -0.0110(15) C5 0.056(2) 0.041(2) 0.049(2) -0.0184(18) 0.0041(18) -0.0133(17) C3 0.078(3) 0.0278(18) 0.055(2) 0.0184(18) 0.018(2) 0.0068(16) O1 0.138(4) 0.059(2) 0.146(4) -0.045(3) -0.002(4) -0.036(2) loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0181 0.0091 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' Cu Cu -1.9646 0.5888 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0311 0.0180 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' O O 0.0492 0.0322 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle _geom_angle_publ_flag O1W Cu1 O1W . 3_666 180.0 ? O1W Cu1 N1 3_666 3_666 87.62(11) ? O1W Cu1 N1 3_666 . 92.38(11) ? O1W Cu1 N1 . 3_666 92.38(11) ? O1W Cu1 N1 . . 87.62(11) ? O1W Cu1 O3 . 3_666 85.93(12) ? O1W Cu1 O3 . . 94.07(12) ? O1W Cu1 O3 3_666 3_666 94.07(12) ? O1W Cu1 O3 3_666 . 85.93(12) ? N1 Cu1 N1 3_666 . 180.0 ? N1 Cu1 O3 3_666 3_666 95.99(11) ? N1 Cu1 O3 . 3_666 84.01(11) ? N1 Cu1 O3 3_666 . 84.01(11) ? N1 Cu1 O3 . . 95.99(11) ? O3 Cu1 O3 3_666 . 180.0 ? Cu1 O1W H1WA . . 117(4) ? Cu1 O1W H1WB . . 116(4) ? H1WA O1W H1WB . . 105(5) ? Cu1 N1 H1A . . 101(3) ? Cu1 N1 H1B . . 100(3) ? C1 N1 Cu1 . . 120.2(2) ? C1 N1 H1A . . 111(3) ? C1 N1 H1B . . 114(3) ? H1A N1 H1B . . 109(4) ? N3 O3 Cu1 . . 122.4(2) ? O4 N3 O3 . . 119.4(3) ? O5 N3 O3 . . 117.8(3) ? O5 N3 O4 . . 122.8(3) ? C6 C1 N1 . . 118.3(3) ? C2 C1 N1 . . 120.8(3) ? C2 C1 C6 . . 120.9(3) ? C1 C6 H6 . . 120.1 ? C5 C6 C1 . . 119.9(3) ? C5 C6 H6 . . 120.1 ? O2 N2 C4 . . 117.7(5) ? O2 N2 O1 . . 124.6(4) ? O1 N2 C4 . . 117.7(5) ? C1 C2 H2 . . 120.6 ? C1 C2 C3 . . 118.7(4) ? C3 C2 H2 . . 120.6 ? C5 C4 N2 . . 118.1(4) ? C5 C4 C3 . . 122.4(3) ? C3 C4 N2 . . 119.5(4) ? C6 C5 H5 . . 120.4 ? C4 C5 C6 . . 119.2(4) ? C4 C5 H5 . . 120.4 ? C2 C3 H3 . . 120.5 ? C4 C3 C2 . . 118.9(4) ? C4 C3 H3 . . 120.5 ? loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_site_symmetry_2 _geom_bond_distance _geom_bond_publ_flag Cu1 O1W . 1.996(2) ? Cu1 O1W 3_666 1.996(2) ? Cu1 N1 . 2.055(3) ? Cu1 N1 3_666 2.055(3) ? Cu1 O3 3_666 2.367(2) ? Cu1 O3 . 2.367(2) ? O1W H1WA . 0.81(6) ? O1W H1WB . 0.76(6) ? N1 C1 . 1.431(4) ? N1 H1A . 0.82(4) ? N1 H1B . 0.86(4) ? O3 N3 . 1.272(4) ? O4 N3 . 1.219(4) ? N3 O5 . 1.217(4) ? C1 C6 . 1.389(5) ? C1 C2 . 1.373(5) ? O2 N2 . 1.209(6) ? C6 H6 . 0.9300 ? C6 C5 . 1.368(5) ? N2 C4 . 1.485(5) ? N2 O1 . 1.229(6) ? C2 H2 . 0.9300 ? C2 C3 . 1.403(5) ? C4 C5 . 1.363(6) ? C4 C3 . 1.367(6) ? C5 H5 . 0.9300 ? C3 H3 . 0.9300 ? loop_ _geom_hbond_atom_site_label_D _geom_hbond_atom_site_label_H _geom_hbond_atom_site_label_A _geom_hbond_site_symmetry_D _geom_hbond_site_symmetry_H _geom_hbond_site_symmetry_A _geom_hbond_distance_DH _geom_hbond_distance_HA _geom_hbond_distance_DA _geom_hbond_angle_DHA _geom_hbond_publ_flag N1 H1A O4 ? ? . 0.82(4) 2.30(4) 3.021(4) 147(4) yes O1W H1WA O3 . . 1_655 0.81(5) 2.07(5) 2.828(4) 156(5) yes O1W H1WA O5 . . 1_655 0.81(5) 2.28(5) 2.979(5) 145(5) yes N1 H1A O4 . . 3_665 0.82(4) 2.42(4) 3.057(4) 135(3) yes N1 H1B O3 . . 1_655 0.86(4) 2.34(4) 3.103(4) 148(4) yes N1 H1B O3 . . 3_666 0.86(4) 2.60(5) 2.968(4) 107(3) yes O1W H1WB O1 . . 2_655 0.76(6) 2.64(5) 3.085(5) 120(5) yes O1W H1WB O2 . . 2_655 0.77(6) 2.26(6) 3.022(5) 171(5) yes loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion _geom_torsion_publ_flag Cu1 N1 C1 C6 . . . . 81.0(3) ? Cu1 N1 C1 C2 . . . . -97.5(3) ? Cu1 O3 N3 O4 . . . . 17.1(4) ? Cu1 O3 N3 O5 . . . . -163.2(3) ? N1 C1 C6 C5 . . . . -178.4(3) ? N1 C1 C2 C3 . . . . 179.2(3) ? C1 C6 C5 C4 . . . . -0.2(6) ? C1 C2 C3 C4 . . . . -1.6(6) ? O2 N2 C4 C5 . . . . 173.9(4) ? O2 N2 C4 C3 . . . . -5.9(6) ? C6 C1 C2 C3 . . . . 0.7(5) ? N2 C4 C5 C6 . . . . 179.5(4) ? N2 C4 C3 C2 . . . . -178.6(4) ? C2 C1 C6 C5 . . . . 0.2(5) ? C5 C4 C3 C2 . . . . 1.6(6) ? C3 C4 C5 C6 . . . . -0.7(6) ? O1 N2 C4 C5 . . . . -5.2(6) ? O1 N2 C4 C3 . . . . 175.0(4) ? _cod_database_fobs_code 2244202